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      Relation between the nodal and antinodal gap and critical temperature in superconducting Bi2212

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          Abstract

          An energy gap is, in principle, a dominant parameter in superconductivity. However, this view has been challenged for the case of high- T c cuprates, because anisotropic evolution of a d-wave-like superconducting gap with underdoping has been difficult to formulate along with a critical temperature T c. Here we show that a nodal-gap energy 2Δ N closely follows 8.5 k B T c with underdoping and is also proportional to the product of an antinodal gap energy Δ * and a square-root superfluid density √ P s for Bi 2Sr 2CaCu 2O 8+ δ , using low-energy synchrotron-radiation angle-resolved photoemission. The quantitative relations imply that the distinction between the nodal and antinodal gaps stems from the separation of the condensation and formation of electron pairs, and that the nodal-gap suppression represents the substantial phase incoherence inherent in a strong-coupling superconducting state. These simple gap-based formulae reasonably describe a crucial part of the unconventional mechanism governing T c.

          Abstract

          In conventional superconductors, the critical temperature is proportional to the superconducting energy gap, but this is not so in unconventional superconductors. Anzai et al. identify an alternative relationship involving nodal and antinodal gaps in an underdoped cuprate superconductor.

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          Most cited references13

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          How Cooper pairs vanish approaching the Mott insulator in Bi2Sr2CaCu2O8+d

          The antiferromagnetic ground state of copper oxide Mott insulators is achieved by localizing an electron at each copper atom in real space (r-space). Removing a small fraction of these electrons (hole doping) transforms this system into a superconducting fluid of delocalized Cooper pairs in momentum space (k-space). During this transformation, two distinctive classes of electronic excitations appear. At high energies, the enigmatic 'pseudogap' excitations are found, whereas, at lower energies, Bogoliubov quasi-particles -- the excitations resulting from the breaking of Cooper pairs -- should exist. To explore this transformation, and to identify the two excitation types, we have imaged the electronic structure of Bi2Sr2CaCu2O8+d in r-space and k-space simultaneously. We find that although the low energy excitations are indeed Bogoliubov quasi-particles, they occupy only a restricted region of k-space that shrinks rapidly with diminishing hole density. Concomitantly, spectral weight is transferred to higher energy r-space states that lack the characteristics of excitations from delocalized Cooper pairs. Instead, these states break translational and rotational symmetries locally at the atomic scale in an energy independent fashion. We demonstrate that these unusual r-space excitations are, in fact, the pseudogap states. Thus, as the Mott insulating state is approached by decreasing the hole density, the delocalized Cooper pairs vanish from k-space, to be replaced by locally translational- and rotational-symmetry-breaking pseudogap states in r-space.
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            Abrupt Onset of Second Energy Gap at Superconducting Transition of Underdoped Bi2212

            The superconducting gap - an energy scale tied to the superconducting phenomena-opens on the Fermi surface at the superconducting transition temperature (TC) in conventional BCS superconductors. Quite differently, in underdoped high-TC superconducting cuprates, a pseudogap, whose relation to the superconducting gap remains a mystery, develops well above TC. Whether the pseudogap is a distinct phenomenon or the incoherent continuation of the superconducting gap above TC is one of the central questions in high-TC research. While some experimental evidence suggests they are distinct, this issue is still under intense debate. A crucial piece of evidence to firmly establish this two-gap picture is still missing: a direct and unambiguous observation of a single-particle gap tied to the superconducting transition as function of temperature. Here we report the discovery of such an energy gap in underdoped Bi2212 in the momentum space region overlooked in previous measurements. Near the diagonal of Cu-O bond direction (nodal direction), we found a gap which opens at TC and exhibits a canonical (BCS-like) temperature dependence accompanied by the appearance of the so-called Bogoliubov quasiparticles, a classical signature of superconductivity. This is in sharp contrast to the pseudogap near the Cu-O bond direction (antinodal region) measured in earlier experiments. The emerging two-gap phenomenon points to a picture of richer quantum configurations in high temperature superconductors.
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              Phase competition in trisected superconducting dome

              A detailed phenomenology of low energy excitations is a crucial starting point for microscopic understanding of complex materials such as the cuprate high temperature superconductors. Because of its unique momentum-space discrimination, angle-resolved photoemission spectroscopy (ARPES) is ideally suited for this task in the cuprates where emergent phases, particularly superconductivity and the pseudogap, have anisotropic gap structure in momentum space. We present a comprehensive doping-and-temperature dependence ARPES study of spectral gaps in Bi\(_2\)Sr\(_2\)CaCu\(_2\)O\(_{8+\delta}\) (Bi-2212), covering much of the superconducting portion of the phase diagram. In the ground state, abrupt changes in near-nodal gap phenomenology give spectroscopic evidence for two potential quantum critical points, p\(=\)0.19 for the pseudogap phase and p\(=\)0.076 for another competing phase. Temperature dependence reveals that the pseudogap is not static below T\(_c\) and exists p\(>\)0.19 at higher temperatures. Our data imply a revised phase diagram which reconciles conflicting reports about the endpoint of the pseudogap in the literature, incorporates phase competition between the superconducting gap and pseudogap, and highlights distinct physics at the edge of the superconducting dome.
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                Author and article information

                Journal
                Nat Commun
                Nat Commun
                Nature Communications
                Nature Pub. Group
                2041-1723
                07 May 2013
                : 4
                : 1815
                Affiliations
                [1 ]Hiroshima Synchrotron Radiation Center, Hiroshima University , Higashi-Hiroshima 739-0046, Japan
                [2 ]Graduate School of Science, Hiroshima University , Higashi-Hiroshima 739-8526, Japan
                [3 ]Department of Physics, University of Tokyo , Tokyo 113-0033, Japan
                [4 ]Laboratory for Atomic and Solid State Physics, Department of Physics, Cornell University , Ithaca, New York 14853, USA
                [5 ]Present address: Graduate School of Engineering, Osaka Prefecture University, Sakai 599-8531, Japan
                [6 ]Present address: Research Center for Neutron Science and Technology, CROSS, Tokai, Ibaraki 319-1106, Japan
                Author notes
                Article
                ncomms2805
                10.1038/ncomms2805
                3674243
                23652003
                0035e7d0-1298-460e-a4a7-5862f3665856
                Copyright © 2013, Nature Publishing Group, a division of Macmillan Publishers Limited. All Rights Reserved.

                This work is licensed under a Creative Commons Attribution-NonCommercial-ShareAlike 3.0 Unported License. To view a copy of this license, visit http://creativecommons.org/licenses/by-nc-sa/3.0/

                History
                : 23 August 2012
                : 24 March 2013
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