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      NASA GEOS Composition Forecast Modeling System GEOS‐CF v1.0: Stratospheric Composition

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          Abstract

          The NASA Goddard Earth Observing System (GEOS) Composition Forecast (GEOS‐CF) provides recent estimates and 5‐day forecasts of atmospheric composition to the public in near‐real time. To do this, the GEOS Earth system model is coupled with the GEOS‐Chem tropospheric‐stratospheric unified chemistry extension (UCX) to represent composition from the surface to the top of the GEOS atmosphere (0.01 hPa). The GEOS‐CF system is described, including updates made to the GEOS‐Chem UCX mechanism within GEOS‐CF for improved representation of stratospheric chemistry. Comparisons are made against balloon, lidar, and satellite observations for stratospheric composition, including measurements of ozone (O 3) and important nitrogen and chlorine species related to stratospheric O 3 recovery. The GEOS‐CF nudges the stratospheric O 3 toward the GEOS Forward Processing (GEOS FP) assimilated O 3 product; as a result the stratospheric O 3 in the GEOS‐CF historical estimate agrees well with observations. During abnormal dynamical and chemical environments such as the 2020 polar vortexes, the GEOS‐CF O 3 forecasts are more realistic than GEOS FP O 3 forecasts because of the inclusion of the complex GEOS‐Chem UCX stratospheric chemistry. Overall, the spatial patterns of the GEOS‐CF simulated concentrations of stratospheric composition agree well with satellite observations. However, there are notable biases—such as low NO x and HNO 3 in the polar regions and generally low HCl throughout the stratosphere—and future improvements to the chemistry mechanism and emissions are discussed. GEOS‐CF is a new tool for the research community and instrument teams observing trace gases in the stratosphere and troposphere, providing near‐real‐time three‐dimensional gridded information on atmospheric composition.

          Key Points

          • Demonstrate the GEOS‐CF system is capable of supporting NASA science missions and applications which observe stratospheric composition

          • The GEOS‐CF model produces realistic stratospheric ozone forecasts, a new capability during anomalous polar vortex conditions

          • Spatial patterns of the GEOS‐CF simulated concentrations of stratospheric composition agree well with independent observations

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          Most cited references132

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          Temporary reduction in daily global CO2 emissions during the COVID-19 forced confinement

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            Large losses of total ozone in Antarctica reveal seasonal ClOx/NOx interaction

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                Author and article information

                Contributors
                k.e.knowland@nasa.gov
                Journal
                J Adv Model Earth Syst
                J Adv Model Earth Syst
                10.1002/(ISSN)1942-2466
                JAME
                Journal of Advances in Modeling Earth Systems
                John Wiley and Sons Inc. (Hoboken )
                1942-2466
                07 June 2022
                June 2022
                : 14
                : 6 ( doiID: 10.1002/jame.v14.6 )
                : e2021MS002852
                Affiliations
                [ 1 ] Universities Space Research Association (USRA)/GESTAR Columbia MD USA
                [ 2 ] NASA Goddard Space Flight Center (GSFC) Global Modeling and Assimilation Office (GMAO) Greenbelt MD USA
                [ 3 ] Now Morgan State University (MSU)/GESTAR‐II Baltimore MD USA
                [ 4 ] Science Systems and Applications (SSAI), Inc. Lanham MD USA
                [ 5 ] Earth Science Division NASA Ames Research Center Moffett Field CA USA
                [ 6 ] Atmospheric Chemistry and Dynamics Laboratory NASA GSFC Greenbelt MD USA
                [ 7 ] Laboratory for Aviation and the Environment Department of Aeronautics and Astronautics Massachusetts Institute of Technology Cambridge MA USA
                [ 8 ] Joint Program on the Science and Policy of Global Change Massachusetts Institute of Technology Cambridge MA USA
                [ 9 ] Jet Propulsion Laboratory California Institute of Technology Wrightwood CA USA
                [ 10 ] Jet Propulsion Laboratory California Institute of Technology Pasadena CA USA
                [ 11 ] Department of Physics University of Toronto Toronto ON Canada
                Author notes
                [*] [* ] Correspondence to:

                K. E. Knowland,

                k.e.knowland@ 123456nasa.gov

                Author information
                https://orcid.org/0000-0003-0837-8502
                https://orcid.org/0000-0002-0552-4298
                https://orcid.org/0000-0002-6445-9254
                https://orcid.org/0000-0002-3795-2983
                https://orcid.org/0000-0002-0414-0882
                https://orcid.org/0000-0002-6010-7497
                https://orcid.org/0000-0003-4419-9157
                https://orcid.org/0000-0002-2476-4801
                https://orcid.org/0000-0003-0880-0232
                https://orcid.org/0000-0002-8430-0515
                https://orcid.org/0000-0001-8753-9153
                https://orcid.org/0000-0003-3420-9454
                https://orcid.org/0000-0002-0035-9625
                https://orcid.org/0000-0003-0200-717X
                Article
                JAME21584 2021MS002852
                10.1029/2021MS002852
                9287101
                052a1f34-6e19-4a6e-a042-e7305ffc595b
                © 2022 The Authors. This article has been contributed to by U.S. Government employees and their work is in the public domain in the USA.

                This is an open access article under the terms of the http://creativecommons.org/licenses/by-nc-nd/4.0/ License, which permits use and distribution in any medium, provided the original work is properly cited, the use is non‐commercial and no modifications or adaptations are made.

                History
                : 03 March 2022
                : 30 September 2021
                : 13 April 2022
                Page count
                Figures: 16, Tables: 2, Pages: 28, Words: 17918
                Funding
                Funded by: National Aeronautics and Space Administration , doi 10.13039/100000104;
                Funded by: NASA Center for Climate Simulation (NCCS)
                Categories
                Atmospheric Composition and Structure
                Middle Atmosphere: Composition and Chemistry
                Middle Atmosphere: Constituent Transport and Chemistry
                Atmospheric Composition and Structure
                Air/Sea Constituent Fluxes
                Middle Atmosphere: Energy Deposition
                Volcanic Effects
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                Gravity and Isostasy
                Atmospheric Processes
                Stratosphere/Troposphere Interactions
                Atmospheric Processes
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                Climatology
                General Circulation
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                Research Article
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                Custom metadata
                2.0
                June 2022
                Converter:WILEY_ML3GV2_TO_JATSPMC version:6.1.7 mode:remove_FC converted:15.07.2022

                geos,ozone,stratosphere,atmospheric chemistry,near real‐time forecasting,global modeling

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