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      Additive interfacial chiral interaction in multilayers for stabilization of small individual skyrmion at room temperature

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          Abstract

          Facing the ever-growing demand for data storage will most probably require a new paradigm. Nanoscale magnetic skyrmions are anticipated to solve this issue as they are arguably the smallest spin textures in magnetic thin films in nature. We designed cobalt-based multilayered thin films where the cobalt layer is sandwiched between two heavy metals providing additive interfacial Dzyaloshinskii-Moriya interactions, which reach a value close to 2 mJ m-2 in the case of the Ir|Co|Pt asymmetric multilayers. Using a magnetization-sensitive scanning x-ray transmission microscopy technique, we imaged small magnetic domains at very low field in these multilayers. The study of their behavior in perpendicular magnetic field allows us to conclude that they are actually magnetic skyrmions stabilized by the large Dzyaloshinskii-Moriya interaction. This discovery of stable sub-100 nm individual skyrmions at room temperature in a technologically relevant material opens the way for device applications in a near future.

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          Real-space observation of a two-dimensional skyrmion crystal.

          Crystal order is not restricted to the periodic atomic array, but can also be found in electronic systems such as the Wigner crystal or in the form of orbital order, stripe order and magnetic order. In the case of magnetic order, spins align parallel to each other in ferromagnets and antiparallel in antiferromagnets. In other, less conventional, cases, spins can sometimes form highly nontrivial structures called spin textures. Among them is the unusual, topologically stable skyrmion spin texture, in which the spins point in all the directions wrapping a sphere. The skyrmion configuration in a magnetic solid is anticipated to produce unconventional spin-electronic phenomena such as the topological Hall effect. The crystallization of skyrmions as driven by thermal fluctuations has recently been confirmed in a narrow region of the temperature/magnetic field (T-B) phase diagram in neutron scattering studies of the three-dimensional helical magnets MnSi (ref. 17) and Fe(1-x)Co(x)Si (ref. 22). Here we report real-space imaging of a two-dimensional skyrmion lattice in a thin film of Fe(0.5)Co(0.5)Si using Lorentz transmission electron microscopy. With a magnetic field of 50-70 mT applied normal to the film, we observe skyrmions in the form of a hexagonal arrangement of swirling spin textures, with a lattice spacing of 90 nm. The related T-B phase diagram is found to be in good agreement with Monte Carlo simulations. In this two-dimensional case, the skyrmion crystal seems very stable and appears over a wide range of the phase diagram, including near zero temperature. Such a controlled nanometre-scale spin topology in a thin film may be useful in observing unconventional magneto-transport effects.
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            Nucleation, stability and current-induced motion of isolated magnetic skyrmions in nanostructures.

            Magnetic skyrmions are topologically stable spin configurations, which usually originate from chiral interactions known as Dzyaloshinskii-Moriya interactions. Skyrmion lattices were initially observed in bulk non-centrosymmetric crystals, but have more recently been noted in ultrathin films, where their existence is explained by interfacial Dzyaloshinskii-Moriya interactions induced by the proximity to an adjacent layer with strong spin-orbit coupling. Skyrmions are promising candidates as information carriers for future information-processing devices due to their small size (down to a few nanometres) and to the very small current densities needed to displace skyrmion lattices. However, any practical application will probably require the creation, manipulation and detection of isolated skyrmions in magnetic thin-film nanostructures. Here, we demonstrate by numerical investigations that an isolated skyrmion can be a stable configuration in a nanostructure, can be locally nucleated by injection of spin-polarized current, and can be displaced by current-induced spin torques, even in the presence of large defects.
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              Skyrmion Lattice in a Chiral Magnet

              Skyrmions represent topologically stable field configurations with particle-like properties. We used neutron scattering to observe the spontaneous formation of a two-dimensional lattice of skyrmion lines, a type of magnetic vortices, in the chiral itinerant-electron magnet MnSi. The skyrmion lattice stabilizes at the border between paramagnetism and long-range helimagnetic order perpendicular to a small applied magnetic field regardless of the direction of the magnetic field relative to the atomic lattice. Our study experimentally establishes magnetic materials lacking inversion symmetry as an arena for new forms of crystalline order composed of topologically stable spin states.
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                Author and article information

                Journal
                2016-07-11
                Article
                10.1038/nnano.2015.313
                1607.02958
                069e32d8-8a8c-42ec-bfee-65f51810c52b

                http://arxiv.org/licenses/nonexclusive-distrib/1.0/

                History
                Custom metadata
                Nature Nanotechnology, Nature Publishing Group, 2016, Graphene bilayers made easy, 11 (5)
                cond-mat.mtrl-sci
                ccsd

                Condensed matter
                Condensed matter

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