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      Development of amidoboranes for hydrogen storage

      , , ,
      Chemical Communications
      Royal Society of Chemistry (RSC)

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          Hydrogen storage in microporous metal-organic frameworks.

          Metal-organic framework-5 (MOF-5) of composition Zn4O(BDC)3 (BDC = 1,4-benzenedicarboxylate) with a cubic three-dimensional extended porous structure adsorbed hydrogen up to 4.5 weight percent (17.2 hydrogen molecules per formula unit) at 78 kelvin and 1.0 weight percent at room temperature and pressure of 20 bar. Inelastic neutron scattering spectroscopy of the rotational transitions of the adsorbed hydrogen molecules indicates the presence of two well-defined binding sites (termed I and II), which we associate with hydrogen binding to zinc and the BDC linker, respectively. Preliminary studies on topologically similar isoreticular metal-organic framework-6 and -8 (IRMOF-6 and -8) having cyclobutylbenzene and naphthalene linkers, respectively, gave approximately double and quadruple (2.0 weight percent) the uptake found for MOF-5 at room temperature and 10 bar.
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            Storage of hydrogen in single-walled carbon nanotubes

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              Complex hydrides for hydrogen storage.

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                Author and article information

                Journal
                CHCOFS
                Chemical Communications
                Chem. Commun.
                Royal Society of Chemistry (RSC)
                1359-7345
                1364-548X
                2011
                2011
                : 47
                : 18
                : 5116
                Article
                10.1039/c0cc05511e
                0d406714-9517-4f23-9de8-119687168959
                © 2011
                History

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