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      Four-Dimensional Scanning Transmission Electron Microscopy (4D-STEM): From Scanning Nanodiffraction to Ptychography and Beyond

      Microscopy and Microanalysis
      Cambridge University Press (CUP)

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          Abstract

          Scanning transmission electron microscopy (STEM) is widely used for imaging, diffraction, and spectroscopy of materials down to atomic resolution. Recent advances in detector technology and computational methods have enabled many experiments that record a full image of the STEM probe for many probe positions, either in diffraction space or real space. In this paper, we review the use of these four-dimensional STEM experiments for virtual diffraction imaging, phase, orientation and strain mapping, measurements of medium-range order, thickness and tilt of samples, and phase contrast imaging methods, including differential phase contrast, ptychography, and others.

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          Topology of covalent non-crystalline solids I: Short-range order in chalcogenide alloys

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            An improved ptychographical phase retrieval algorithm for diffractive imaging.

            The ptychographical iterative engine (or PIE) is a recently developed phase retrieval algorithm that employs a series of diffraction patterns recorded as a known illumination function is translated to a set of overlapping positions relative to a target sample. The technique has been demonstrated successfully at optical and X-ray wavelengths and has been shown to be robust to detector noise and to converge considerably faster than support-based phase retrieval methods. In this paper, the PIE is extended so that the requirement for an accurate model of the illumination function is removed.
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              The scattering of electrons by atoms and crystals. I. A new theoretical approach

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                Author and article information

                Journal
                Microscopy and Microanalysis
                Microsc Microanal
                Cambridge University Press (CUP)
                1431-9276
                1435-8115
                June 2019
                May 14 2019
                June 2019
                : 25
                : 3
                : 563-582
                Article
                10.1017/S1431927619000497
                31084643
                128260b9-7e01-43b5-bc95-eed727f008a1
                © 2019

                https://www.cambridge.org/core/terms

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