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      The future of low-temperature carbon dioxide electrolysis depends on solving one basic problem

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      Author(s): ,
      Publication date (Electronic):
      Journal: Nature Communications
      Publisher: Nature Publishing Group UK
      Keywords: Electrocatalysis, Energy, Electrocatalysis

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          Abstract

          Carbonate formation is the primary source of energy and carbon losses in low-temperature carbon dioxide electrolysis. Realigning research priorities to address the carbonate problem is essential if this technology is to become a viable option for renewable chemical and fuel production.

          Abstract

          Low-temperature carbon dioxide electrolysis is an attractive process for sustainable fuel synthesis, but current systems suffer from low efficiency. In this comment, authors discuss the limitations arising from the reaction between carbon dioxide and hydroxide, highlighting the need for new research to address this fundamental problem.

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          Double-slit photoelectron interference in strong-field ionization of the neon dimer

          Maksim Kunitski, Nicolas Eicke, Pia Huber … (2019)
          Wave-particle duality is an inherent peculiarity of the quantum world. The double-slit experiment has been frequently used for understanding different aspects of this fundamental concept. The occurrence of interference rests on the lack of which-way information and on the absence of decoherence mechanisms, which could scramble the wave fronts. Here, we report on the observation of two-center interference in the molecular-frame photoelectron momentum distribution upon ionization of the neon dimer by a strong laser field. Postselection of ions, which are measured in coincidence with electrons, allows choosing the symmetry of the residual ion, leading to observation of both, gerade and ungerade, types of interference.
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            CO2electroreduction to ethylene via hydroxide-mediated copper catalysis at an abrupt interface

            Christine M Gabardo, F García de Arquer, Amirreza Kiani … (2018)
            Article 0 comments Cited 809 times – based on 0 reviews     Review now
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              CO2 electrolysis to multicarbon products at activities greater than 1 A cm−2

              F García de Arquer, Cao-Thang Dinh, Adnan Ozden … (2020)
              Electrolysis offers an attractive route to upgrade greenhouse gases such as carbon dioxide (CO 2 ) to valuable fuels and feedstocks; however, productivity is often limited by gas diffusion through a liquid electrolyte to the surface of the catalyst. Here, we present a catalyst:ionomer bulk heterojunction (CIBH) architecture that decouples gas, ion, and electron transport. The CIBH comprises a metal and a superfine ionomer layer with hydrophobic and hydrophilic functionalities that extend gas and ion transport from tens of nanometers to the micrometer scale. By applying this design strategy, we achieved CO 2 electroreduction on copper in 7 M potassium hydroxide electrolyte (pH ≈ 15) with an ethylene partial current density of 1.3 amperes per square centimeter at 45% cathodic energy efficiency.
              Article 0 comments Cited 477 times – based on 0 reviews     Review now
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                Author and article information

                Contributors
                Matthew W. Kanan:
                ORCID: http://orcid.org/0000-0002-5932-6289
                mkanan@stanford.edu
                Journal
                Journal ID (nlm-ta): Nat Commun
                Journal ID (iso-abbrev): Nat Commun
                Title: Nature Communications
                Publisher: Nature Publishing Group UK (London )
                ISSN (Electronic): 2041-1723
                Publication date (Electronic): 16 October 2020
                Publication date PMC-release: 16 October 2020
                Publication date Collection: 2020
                Volume: 11
                Electronic Location Identifier: 5231
                Affiliations
                GRID grid.168010.e, ISNI 0000000419368956, Department of Chemistry, , Stanford University, ; 337 Campus Drive, Stanford, CA 94305 USA
                Author information
                http://orcid.org/0000-0001-9330-0464
                http://orcid.org/0000-0002-5932-6289
                Article
                Publisher ID: 19135
                DOI: 10.1038/s41467-020-19135-8
                PMC ID: 7567821
                PubMed ID: 33067444
                SO-VID: 21222867-71e5-4770-8bd4-b7666d182ec3
                Copyright © © The Author(s) 2020
                License:

                Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.

                History
                Date received : 31 August 2020
                Date accepted : 25 September 2020
                Categories
                Subject: Comment
                Custom metadata
                issue-copyright-statement © The Author(s) 2020

                ScienceOpen disciplines: Uncategorized
                Keywords: electrocatalysis,energy
                Data availability:
                ScienceOpen disciplines: Uncategorized
                Keywords: electrocatalysis, energy

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