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      Life cycle assessment of carbon dioxide removal technologies: a critical review

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          Abstract

          This review provides a perspective on how to conduct future Life Cycle Assessment (LCA) studies of carbon dioxide removal technologies in a consistent way avoiding common mistakes, which should be addressed to aid informed decision making.

          Abstract

          A large number of prospective climate scenarios rely on Carbon Dioxide Removal (CDR) technologies to limit global warming below 2 °C. To date, however, a comprehensive understanding of the overall life-cycle environmental impacts of CDR technologies is missing. We present a critical review on conducted Life Cycle Assessments (LCAs) of a comprehensive set of CDR technologies: afforestation and reforestation, biochar, soil carbon sequestration, enhanced weathering, ocean fertilisation, bioenergy with carbon capture and storage, and direct air carbon capture and storage. One of the key observations is that emissions avoided due to substitution of certain processes (due to system expansion in LCA) can be easily misinterpreted as negative emissions, i.e. as carbon removal from the atmosphere. Based on the observed inconsistencies and shortcomings, we recommend to interpret available CDR LCA results with caution. To improve the understanding of environmental implications of CDR deployment, we recommend (1) to conduct LCAs with multiple environmental impact categories, (2) to consider the temporal aspect of emissions in biomass-related CDR technologies, (3) to focus on so far overlooked CDR technologies, (4) to be as transparent as possible regarding methodological choices, (5) to capture environmental side-effects, and (6) to distinguish between ‘avoided emissions’ and ‘negative emissions’ – only negative emissions correspond to permanent removal from the atmosphere. We conclude that more comprehensive and rigorous LCAs are needed to help inform the design of CDR technology portfolios and to aid in anticipatory governance.

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          Double-slit photoelectron interference in strong-field ionization of the neon dimer

          Wave-particle duality is an inherent peculiarity of the quantum world. The double-slit experiment has been frequently used for understanding different aspects of this fundamental concept. The occurrence of interference rests on the lack of which-way information and on the absence of decoherence mechanisms, which could scramble the wave fronts. Here, we report on the observation of two-center interference in the molecular-frame photoelectron momentum distribution upon ionization of the neon dimer by a strong laser field. Postselection of ions, which are measured in coincidence with electrons, allows choosing the symmetry of the residual ion, leading to observation of both, gerade and ungerade, types of interference.
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            Structural absorption by barbule microstructures of super black bird of paradise feathers

            Many studies have shown how pigments and internal nanostructures generate color in nature. External surface structures can also influence appearance, such as by causing multiple scattering of light (structural absorption) to produce a velvety, super black appearance. Here we show that feathers from five species of birds of paradise (Aves: Paradisaeidae) structurally absorb incident light to produce extremely low-reflectance, super black plumages. Directional reflectance of these feathers (0.05–0.31%) approaches that of man-made ultra-absorbent materials. SEM, nano-CT, and ray-tracing simulations show that super black feathers have titled arrays of highly modified barbules, which cause more multiple scattering, resulting in more structural absorption, than normal black feathers. Super black feathers have an extreme directional reflectance bias and appear darkest when viewed from the distal direction. We hypothesize that structurally absorbing, super black plumage evolved through sensory bias to enhance the perceived brilliance of adjacent color patches during courtship display.
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              The Shared Socioeconomic Pathways and their energy, land use, and greenhouse gas emissions implications: An overview

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                Author and article information

                Contributors
                Journal
                EESNBY
                Energy & Environmental Science
                Energy Environ. Sci.
                Royal Society of Chemistry (RSC)
                1754-5692
                1754-5706
                April 21 2021
                2021
                : 14
                : 4
                : 1701-1721
                Affiliations
                [1 ]Paul Scherrer Institut
                [2 ]Laboratory for Energy Systems Analysis
                [3 ]5232 Villigen PSI
                [4 ]Switzerland
                [5 ]Institute of Energy and Process Engineering
                [6 ]ETH Zürich
                [7 ]Zürich 8092
                Article
                10.1039/D0EE03757E
                2a9463f2-6688-4d2b-b1fb-73cdb9fdc2d5
                © 2021

                http://creativecommons.org/licenses/by-nc/3.0/

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