Quantum simulation of molecular vibronic spectra on a superconducting
  bosonic processor

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Abstract

The efficient simulation of quantum systems is a primary motivating factor for developing controllable quantum machines. A controllable bosonic machine is naturally suited for simulating systems with underlying bosonic structure, exploiting both quantum interference and an intrinsically large Hilbert space. Here, we experimentally realize a bosonic superconducting processor that combines arbitrary state preparation, a complete set of Gaussian operations, plus an essential non-Gaussian resource - a novel single-shot photon number resolving measurement scheme - all in one device. We utilize these controls to simulate the bosonic problem of molecular vibronic spectra, extracting the corresponding Franck-Condon factors for photoelectron processes in H2O, O3, NO2, and SO2. Our results demonstrate the versatile capabilities of the circuit QED platform, which can be extended to include non-Gaussian operations for simulating an even wider class of bosonic systems.

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Most cited references 12

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Resolving photon number states in a superconducting circuit

D. I. Schuster, A. A. Houck, J. A. Schreier … (2007)

Electromagnetic signals are always composed of photons, although in the circuit domain those signals are carried as voltages and currents on wires, and the discreteness of the photon's energy is usually not evident. However, by coupling a superconducting quantum bit (qubit) to signals on a microwave transmission line, it is possible to construct an integrated circuit in which the presence or absence of even a single photon can have a dramatic effect. Such a system can be described by circuit quantum electrodynamics (QED)-the circuit equivalent of cavity QED, where photons interact with atoms or quantum dots. Previously, circuit QED devices were shown to reach the resonant strong coupling regime, where a single qubit could absorb and re-emit a single photon many times. Here we report a circuit QED experiment in the strong dispersive limit, a new regime where a single photon has a large effect on the qubit without ever being absorbed. The hallmark of this strong dispersive regime is that the qubit transition energy can be resolved into a separate spectral line for each photon number state of the microwave field. The strength of each line is a measure of the probability of finding the corresponding photon number in the cavity. This effect is used to distinguish between coherent and thermal fields, and could be used to create a photon statistics analyser. As no photons are absorbed by this process, it should be possible to generate non-classical states of light by measurement and perform qubit-photon conditional logic, the basis of a logic bus for a quantum computer.

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Confining the state of light to a quantum manifold by engineered two-photon loss

Z Leghtas, S. Touzard, I. Pop … (2015)

Physical systems usually exhibit quantum behavior, such as superpositions and entanglement, only when they are sufficiently decoupled from a lossy environment. Paradoxically, a specially engineered interaction with the environment can become a resource for the generation and protection of quantum states. This notion can be generalized to the confinement of a system into a manifold of quantum states, consisting of all coherent superpositions of multiple stable steady states. We have confined the state of a superconducting resonator to the quantum manifold spanned by two coherent states of opposite phases and have observed a Schrödinger cat state spontaneously squeeze out of vacuum before decaying into a classical mixture. This experiment points toward robustly encoding quantum information in multidimensional steady-state manifolds.