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      Simultaneous atmospheric water production and 24-hour power generation enabled by moisture-induced energy harvesting

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          Abstract

          Water and electricity scarcity are two global challenges, especially in arid and remote areas. Harnessing ubiquitous moisture and sunlight for water and power generation is a sustainable route to address these challenges. Herein, we report a moisture-induced energy harvesting strategy to realize efficient sorption-based atmospheric water harvesting (SAWH) and 24-hour thermoelectric power generation (TEPG) by synergistically utilizing moisture-induced sorption/desorption heats of SAWH, solar energy in the daytime and radiative cooling in the nighttime. Notably, the synergistic effects significantly improve all-day thermoelectric power density (~346%) and accelerate atmospheric water harvesting compared with conventional designs. We further demonstrate moisture-induced energy harvesting for a hybrid SAWH-TEPG device, exhibiting high water production of 750 g m −2, together with impressive thermoelectric power density up to 685 mW m −2 in the daytime and 21 mW m −2 in the nighttime. Our work provides a promising approach to realizing sustainable water production and power generation at anytime and anywhere.

          Abstract

          Collecting water directly from air provides one sustainable solution to water scarcity. Li et al. combine sorption-based atmospheric water harvesting with a thermoelectric module for efficient harvesting water and electricity in arid environments and show that the two components operate synergistically.

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          Most cited references52

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          Four billion people facing severe water scarcity

          Global water scarcity assessment at a high spatial and temporal resolution, accounting for environmental flow requirements.
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            A chromium terephthalate-based solid with unusually large pore volumes and surface area.

            We combined targeted chemistry and computational design to create a crystal structure for porous chromium terephthalate, MIL-101, with very large pore sizes and surface area. Its zeotype cubic structure has a giant cell volume (approximately 702,000 cubic angstroms), a hierarchy of extra-large pore sizes (approximately 30 to 34 angstroms), and a Langmuir surface area for N2 of approximately 5900 +/- 300 square meters per gram. Beside the usual properties of porous compounds, this solid has potential as a nanomold for monodisperse nanomaterials, as illustrated here by the incorporation of Keggin polyanions within the cages.
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              Solar-driven interfacial evaporation

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                Author and article information

                Contributors
                Litx@sjtu.edu.cn
                Journal
                Nat Commun
                Nat Commun
                Nature Communications
                Nature Publishing Group UK (London )
                2041-1723
                9 November 2022
                9 November 2022
                2022
                : 13
                : 6771
                Affiliations
                [1 ]GRID grid.16821.3c, ISNI 0000 0004 0368 8293, Institute of Refrigeration and Cryogenics, School of Mechanical Engineering, , Shanghai Jiao Tong University, ; Shanghai, 200240 China
                [2 ]GRID grid.16821.3c, ISNI 0000 0004 0368 8293, Research Center of Solar Power and Refrigeration of Ministry of Education, , Shanghai Jiao Tong University, ; Shanghai, 200240 China
                Author information
                http://orcid.org/0000-0003-4618-8144
                http://orcid.org/0000-0002-8913-9783
                http://orcid.org/0000-0003-0702-7823
                http://orcid.org/0000-0003-3586-5728
                Article
                34385
                10.1038/s41467-022-34385-4
                9646691
                36351950
                422fbd83-75d1-4178-b705-00db3264c8c2
                © The Author(s) 2022

                Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.

                History
                : 17 April 2022
                : 24 October 2022
                Funding
                Funded by: FundRef https://doi.org/10.13039/501100001809, National Natural Science Foundation of China (National Science Foundation of China);
                Award ID: 51876117
                Award Recipient :
                Categories
                Article
                Custom metadata
                © The Author(s) 2022

                Uncategorized
                devices for energy harvesting,thermoelectric devices and materials,solar thermal energy

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