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      Changes of absorbed dose rate in air in metropolitan Tokyo relating to radiocesium released from the Fukushima Daiichi Nuclear Power Plant accident: Results of a five-year study

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          Abstract

          Car-borne surveys were carried out in metropolitan Tokyo, Japan, in 2015, 2016, 2017 and 2018 to estimate the transition of absorbed dose rate in air from the Fukushima Daiichi Nuclear Power Plant accident. Additionally, the future transition of absorbed dose rates in air based on this five-year study and including previously reported measurements done in 2014 by the authors was analyzed because central Tokyo has large areas covered with asphalt and concrete. The average absorbed dose rate in air (range) in the whole area of Tokyo measured in 2018 was 59 ± 9 nGy h -1 (28–105 nGy h -1), and it was slightly decreased compared to the previously reported value measured in 2011 (61 nGy h -1; 30–200 nGy h -1). In the detailed dose rate distribution map, while areas of higher dose rates exceeding 70 nGy h -1 had been observed on the eastern and western ends of Tokyo after 2014, the dose rates in these areas have decreased yearly. Especially, the decreasing dose rate from radiocesium (Cs-134 + Cs-137) in the eastern end of Tokyo which is mainly covered by asphalt was higher than that measured in the western end which is mainly covered by forest. The percent reductions for the eastern end in the years 2014–2015, 2015–2016, 2016–2017 and 2017–2018 were 49%, 21%, 18% and 16%, and those percent reductions for western end were 26%, 18%, 6% and 3%, respectively. Additionally, the decrease for dose rate from radiocesium depended on the types of asphalt, and that on porous asphalt was larger than the decrease on standard asphalt.

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          Assessment of individual radionuclide distributions from the Fukushima nuclear accident covering central-east Japan.

          A tremendous amount of radioactivity was discharged because of the damage to cooling systems of nuclear reactors in the Fukushima No. 1 nuclear power plant in March 2011. Fukushima and its adjacent prefectures were contaminated with fission products from the accident. Here, we show a geographical distribution of radioactive iodine, tellurium, and cesium in the surface soils of central-east Japan as determined by gamma-ray spectrometry. Especially in Fukushima prefecture, contaminated area spreads around Iitate and Naka-Dori for all the radionuclides we measured. Distributions of the radionuclides were affected by the physical state of each nuclide as well as geographical features. Considering meteorological conditions, it is concluded that the radioactive material transported on March 15 was the major contributor to contamination in Fukushima prefecture, whereas the radioactive material transported on March 21 was the major source in Ibaraki, Tochigi, Saitama, and Chiba prefectures and in Tokyo.
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            Atmospheric behavior, deposition, and budget of radioactive materials from the Fukushima Daiichi nuclear power plant in March 2011

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              Detailed deposition density maps constructed by large-scale soil sampling for gamma-ray emitting radioactive nuclides from the Fukushima Dai-ichi Nuclear Power Plant accident.

              Soil deposition density maps of gamma-ray emitting radioactive nuclides from the Fukushima Dai-ichi Nuclear Power Plant (NPP) accident were constructed on the basis of results from large-scale soil sampling. In total 10,915 soil samples were collected at 2168 locations. Gamma rays emitted from the samples were measured by Ge detectors and analyzed using a reliable unified method. The determined radioactivity was corrected to that of June 14, 2011 by considering the intrinsic decay constant of each nuclide. Finally the deposition maps were created for (134)Cs, (137)Cs, (131)I, (129m)Te and (110m)Ag. The radioactivity ratio of (134)Cs-(137)Cs was almost constant at 0.91 regardless of the locations of soil sampling. The radioactivity ratios of (131)I and (129m)Te-(137)Cs were relatively high in the regions south of the Fukushima NPP site. Effective doses for 50 y after the accident were evaluated for external and inhalation exposures due to the observed radioactive nuclides. The radiation doses from radioactive cesium were found to be much higher than those from the other radioactive nuclides.
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                Author and article information

                Contributors
                Role: ConceptualizationRole: Data curationRole: Formal analysisRole: Funding acquisitionRole: Project administrationRole: Writing – original draft
                Role: Data curation
                Role: Data curation
                Role: Data curationRole: Formal analysis
                Role: Data curation
                Role: Data curationRole: Formal analysis
                Role: Data curation
                Role: Data curation
                Role: Formal analysis
                Role: ConceptualizationRole: Data curationRole: Funding acquisitionRole: Writing – original draft
                Role: Editor
                Journal
                PLoS One
                PLoS ONE
                plos
                plosone
                PLoS ONE
                Public Library of Science (San Francisco, CA USA )
                1932-6203
                24 October 2019
                2019
                : 14
                : 10
                : e0224449
                Affiliations
                [1 ] Department of Radiological Sciences, Graduate School of Human Health Sciences, Tokyo Metropolitan University, Arakawa-ku, Tokyo, Japan
                [2 ] Department of Radiological Sciences, Tsukuba International University, Tsuchiura, Ibaraki, Japan
                Fukushima Medical University School of Medicine, JAPAN
                Author notes

                Competing Interests: The authors have declared that no competing interests exist.

                Author information
                http://orcid.org/0000-0003-1292-6364
                Article
                PONE-D-19-17982
                10.1371/journal.pone.0224449
                6812831
                31648245
                488a1a1c-074b-423a-8931-44a7988d15c5
                © 2019 Inoue et al

                This is an open access article distributed under the terms of the Creative Commons Attribution License, which permits unrestricted use, distribution, and reproduction in any medium, provided the original author and source are credited.

                History
                : 28 June 2019
                : 14 October 2019
                Page count
                Figures: 9, Tables: 1, Pages: 15
                Funding
                This work was funded by the strategic research fund of Tokyo Metropolitan University (2015 – 2018).
                Categories
                Research Article
                Biology and Life Sciences
                Biophysics
                Dosimetry
                Physical Sciences
                Physics
                Biophysics
                Dosimetry
                Research and Analysis Methods
                Research Design
                Survey Research
                Surveys
                Earth Sciences
                Geography
                Geographic Areas
                Urban Areas
                Physical Sciences
                Materials Science
                Materials
                Dust
                Physical Sciences
                Physics
                Nuclear Physics
                Nuclear Power
                Physical Sciences
                Materials Science
                Materials
                Porous Materials
                Earth sciences
                Marine and aquatic sciences
                Bodies of water
                Oceans
                Pacific Ocean
                Earth Sciences
                Geomorphology
                Topography
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                All relevant data are within the paper and its Supporting Information files.

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