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      State of the Art in Alcohol Sensing with 2D Materials

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          Highlights

          • A current review on the applications of graphene and other two-dimensional (2D) materials in alcohol detection.

          • A thorough discussion on the fundamental principles and the advantages of using 2D materials in sensing alcohol.

          • Critical discussion of the current limitations of alcohol sensors and the role of 2D materials in addressing the challenges.

          Abstract

          Since the discovery of graphene, the star among new materials, there has been a surge of attention focused on the monatomic and monomolecular sheets which can be obtained by exfoliation of layered compounds. Such materials are known as two-dimensional (2D) materials and offer enormous versatility and potential. The ultimate single atom, or molecule, thickness of the 2D materials sheets provides the highest surface to weight ratio of all the nanomaterials, which opens the door to the design of more sensitive and reliable chemical sensors. The variety of properties and the possibility of tuning the chemical and surface properties of the 2D materials increase their potential as selective sensors, targeting chemical species that were previously difficult to detect. The planar structure and the mechanical flexibility of the sheets allow new sensor designs and put 2D materials at the forefront of all the candidates for wearable applications. When developing sensors for alcohol, the response time is an essential factor for many industrial and forensic applications, particularly when it comes to hand-held devices. Here, we review recent developments in the applications of 2D materials in sensing alcohols along with a study on parameters that affect the sensing capabilities. The review also discusses the strategies used to develop the sensor along with their mechanisms of sensing and provides a critique of the current limitations of 2D materials-based alcohol sensors and an outlook for the future research required to overcome the challenges.

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          Most cited references280

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          Electric Field Effect in Atomically Thin Carbon Films

          We describe monocrystalline graphitic films, which are a few atoms thick but are nonetheless stable under ambient conditions, metallic, and of remarkably high quality. The films are found to be a two-dimensional semimetal with a tiny overlap between valence and conductance bands, and they exhibit a strong ambipolar electric field effect such that electrons and holes in concentrations up to 10 13 per square centimeter and with room-temperature mobilities of ∼10,000 square centimeters per volt-second can be induced by applying gate voltage.
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            Two-dimensional nanocrystals produced by exfoliation of Ti3 AlC2.

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              Preparation of Graphitic Oxide

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                Author and article information

                Contributors
                rboroujerdi@bournemouth.ac.uk
                aa494@cam.ac.uk
                rpaul@bournemouth.ac.uk
                Journal
                Nanomicro Lett
                Nanomicro Lett
                Nano-Micro Letters
                Springer Singapore (Singapore )
                2311-6706
                2150-5551
                21 January 2020
                21 January 2020
                December 2020
                : 12
                : 33
                Affiliations
                [1 ]GRID grid.17236.31, ISNI 0000 0001 0728 4630, Faculty of Science and Technology, , Bournemouth University, Talbot Campus, ; Fern Barrow, Poole, BH12 5BB UK
                [2 ]GRID grid.5335.0, ISNI 0000000121885934, Department of Engineering, , University of Cambridge, ; Cambridge, CB3 0FS UK
                Article
                363
                10.1007/s40820-019-0363-0
                7770777
                4c89de6d-5cae-462e-afc9-840d91d96230
                © The Author(s) 2020

                Open AccessThis article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/.

                History
                : 9 October 2019
                : 5 December 2019
                Categories
                Review
                Custom metadata
                © The Author(s) 2020

                sensors and biosensors,alcohol probes,electrochemical detectors,ethanol metabolites,2d materials

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