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      Aerobic Oxidative Coupling of Resveratrol and its Analogues by Visible Light Using Mesoporous Graphitic Carbon Nitride (mpg-C3N4) as a Bioinspired Catalyst

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          Abstract

          The first aerobic oxidative coupling of resveratrol and its analogues by mesoporous graphitic carbon nitride as a bioinspired catalyst with visible light has been developed. With this method, δ-viniferin and its analogues were synthesized in moderate to high yield. The metal-free conditions, visible-light irradiation, and the ideal oxidant, molecular oxygen, make this coupling reaction environmental friendly and practical.

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          mpg-C(3)N(4)-Catalyzed selective oxidation of alcohols using O(2) and visible light.

          Mesoporous carbon nitride (mpg-C(3)N(4)) polymer can function as a metal-free photocatalyst to activate O(2) for the selective oxidation of benzyl alcohols with visible light, avoiding the cost, toxicity, and purification problems associated with corresponding transition-metal systems. By combining the surface basicity and semiconductor functions of mpg-C(3)N(4), the photocatalytic system can realize a high catalytic selectivity to generate benzaldehyde. The metal-free photocatalytic system also selectively converts other alcohol substrates to their corresponding aldehydes/ketones, demonstrating a potential pathway of accessing traditional mild radical chemistry with nitroxyl radicals.
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            Polymeres graphitisches Kohlenstoffnitrid als heterogener Organokatalysator: von der Photochemie über die Vielzweckkatalyse hin zur nachhaltigen Chemie

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              A new class of phytoalexins from grapevines.

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                Author and article information

                Journal
                Chemistry - A European Journal
                Chem. Eur. J.
                Wiley
                09476539
                January 13 2014
                January 13 2014
                December 04 2013
                : 20
                : 3
                : 678-682
                Article
                10.1002/chem.201303587
                24307535
                4d47adc9-9635-4054-b326-b5d63905663b
                © 2013

                http://doi.wiley.com/10.1002/tdm_license_1.1

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                Self URI (article page): http://doi.wiley.com/10.1002/chem.201303587

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