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      A Robust Porphyrin‐Stabilized Triplet Carbon Diradical

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          Anomalous Paramagnetism of Copper Acetate

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            Highly regioselective Ir-catalyzed beta-borylation of porphyrins via C-H bond activation and construction of beta-beta-linked diporphyrin.

            Highly regioselective borylation of 5,15-diaryl- and 5,10,15-triarylporphyrins has been achieved by the reaction with bis(pinacolato)diborane under iridium catalysis. Borylated porphyrins are a useful building block for constructing porphyrin arrays, hence offering an effective route to beta-functionalized porphyrins.
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              High-spin organic molecules.

              Organic molecules with high-spin ground states, besides being fundamentally interesting, possess numerous potential applications in diverse fields such organic magnetism, MRI contrast agents, and spintronics. Such molecules, once thought to exist only as highly reactive intermediates, can be rationally designed to have adequate stability for organic synthesis and characterization. This Synopsis provides an overview of the factors that lead to high-spin ground states as well as recent progress in the design and synthesis of high-spin organic molecules.
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                Author and article information

                Contributors
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                Journal
                Angewandte Chemie International Edition
                Angew. Chem. Int. Ed.
                Wiley
                1433-7851
                1521-3773
                March 22 2021
                February 24 2021
                March 22 2021
                : 60
                : 13
                : 7002-7006
                Affiliations
                [1 ]College of Chemistry and Chemical Engineering Key Laboratory of Chemical Biology and Traditional Chinese Medicine Research (Ministry of Education of China) Key Laboratory of the Assembly and Application of Organic Functional molecules of Hunan Province Hunan Normal University Changsha 410081 China
                [2 ]Department of Chemistry Graduate School of Science Kyoto University Sakyo-ku Kyoto 606-8502 Japan
                [3 ]Center for Instrumental Analysis Niigata University Nishi-ku Niigata 950-2181 Japan
                Article
                10.1002/anie.202015356
                4faccae5-6a7c-4821-a460-5b5278382205
                © 2021

                http://onlinelibrary.wiley.com/termsAndConditions#vor

                http://doi.wiley.com/10.1002/tdm_license_1.1

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