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      Incipient charge order observed by NMR in the normal state of YBa 2Cu 3O y

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          Abstract

          The pseudogap regime of high-temperature cuprates harbours diverse manifestations of electronic ordering whose exact nature and universality remain debated. Here, we show that the short-ranged charge order recently reported in the normal state of YBa 2Cu 3O y corresponds to a truly static modulation of the charge density. We also show that this modulation impacts on most electronic properties, that it appears jointly with intra-unit-cell nematic, but not magnetic, order, and that it exhibits differences with the charge density wave observed at lower temperatures in high magnetic fields. These observations prove mostly universal, they place new constraints on the origin of the charge density wave and they reveal that the charge modulation is pinned by native defects. Similarities with results in layered metals such as NbSe 2, in which defects nucleate halos of incipient charge density wave at temperatures above the ordering transition, raise the possibility that order–parameter fluctuations, but no static order, would be observed in the normal state of most cuprates if disorder were absent.

          Abstract

          The nature and universality of the ordering phenomena observed in the normal state of high-temperature superconductors remain unclear. Here, Wu et al. observe several aspects of incipient charge ordering in YBCO via NMR measurements, clarifying the role of quenched disorder in their emergence.

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          Most cited references31

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          Long-range incommensurate charge fluctuations in (Y,Nd)Ba2Cu3O(6+x)

          There are increasing indications that superconductivity competes with other orders in cuprate superconductors, but obtaining direct evidence with bulk-sensitive probes is challenging. We have used resonant soft x-ray scattering to identify two-dimensional charge fluctuations with an incommensurate periodicity of \(\bf \sim 3.2\) lattice units in the copper-oxide planes of the superconductors (Y,Nd)Ba\(_2\)Cu\(_3\)O\(_{6+x}\) with hole concentrations \(0.09 \leq p \leq 0.13\) per planar Cu ion. The intensity and correlation length of the fluctuation signal increase strongly upon cooling down to the superconducting transition temperature, \(T_c\); further cooling below \(T_c\) abruptly reverses the divergence of the charge correlations. In combination with prior observations of a large gap in the spin excitation spectrum, these data indicate an incipient charge-density-wave instability that competes with superconductivity.
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            Electron pockets in the Fermi surface of hole-doped high-Tc superconductors

            High-temperature superconductivity occurs as copper oxides are chemically tuned to have a carrier concentration intermediate between their metallic state at high doping and their insulating state at zero doping. The underlying evolution of the electron system in the absence of superconductivity is still unclear and a question of central importance is whether it involves any intermediate phase with broken symmetry. The Fermi surface of underdoped YBa2Cu3Oy and YBa2Cu4O8 was recently shown to include small pockets in contrast with the large cylinder characteristic of the overdoped regime1, pointing to a topological change in the Fermi surface. Here we report the observation of a negative Hall resistance in the magnetic field-induced normal state of YBa2Cu3Oy and YBa2Cu4O8, which reveals that these pockets are electron-like. We propose that electron pockets arise most likely from a reconstruction of the Fermi surface caused by the onset of a density-wave phase, as is thought to occur in the electron-doped materials near the onset of antiferromagnetic order Comparison with materials of the La2CuO4 family that exhibit spin/charge density-wave order suggests that a Fermi surface reconstruction also occurs in those materials, pointing to a generic property of high-Tc superconductors.
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              Magnetic-field-induced charge-stripe order in the high temperature superconductor YBa2Cu3Oy

              Electronic charges introduced in copper-oxide planes generate high-transition temperature superconductivity but, under special circumstances, they can also order into filaments called stripes. Whether an underlying tendency of charges to order is present in all cuprates and whether this has any relationship with superconductivity are, however, two highly controversial issues. In order to uncover underlying electronic orders, magnetic fields strong enough to destabilise superconductivity can be used. Such experiments, including quantum oscillations in YBa2Cu3Oy (a notoriously clean cuprate where charge order is not observed) have suggested that superconductivity competes with spin, rather than charge, order. Here, using nuclear magnetic resonance, we demonstrate that high magnetic fields actually induce charge order, without spin order, in the CuO2 planes of YBa2Cu3Oy. The observed static, unidirectional, modulation of the charge density breaks translational symmetry, thus explaining quantum oscillation results, and we argue that it is most likely the same 4a-periodic modulation as in stripe-ordered cuprates. The discovery that it develops only when superconductivity fades away and near the same 1/8th hole doping as in La2-xBaxCuO4 suggests that charge order, although visibly pinned by CuO chains in YBa2Cu3Oy, is an intrinsic propensity of the superconducting planes of high Tc cuprates.
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                Author and article information

                Journal
                Nat Commun
                Nat Commun
                Nature Communications
                Nature Pub. Group
                2041-1723
                09 March 2015
                : 6
                : 6438
                Affiliations
                [1 ]Laboratoire National des Champs Magnétiques Intenses, UPR 3228, CNRS-UJF-UPS-INSA , 38042 Grenoble, France
                [2 ]Department of Physics and Astronomy, University of British Columbia , Vancouver, British Columbia, Canada V6T 1Z1
                [3 ]Canadian Institute for Advanced Research , Toronto, Ontario, Canada M5G 1Z8
                Author notes
                [*]

                Present address: Hefei National Laboratory for Physical Sciences at Microscale, University of Science and Technology of China, No. 96 Jinzhai Road, Hefei 230026, P.R. China

                Article
                ncomms7438
                10.1038/ncomms7438
                4366503
                25751448
                5310d180-2b23-4cff-8693-65036994cc7f
                Copyright © 2015, Nature Publishing Group, a division of Macmillan Publishers Limited. All Rights Reserved.

                This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/

                History
                : 09 January 2015
                : 28 January 2015
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