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      Multiflat Bands and Strong Correlations in Twisted Bilayer Boron Nitride: Doping-Induced Correlated Insulator and Superconductor

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          Abstract

          Two-dimensional materials, obtained by van der Waals stacking of layers, are fascinating objects of contemporary condensed matter research, exhibiting a variety of new physics. Inspired by the breakthroughs of twisted bilayer graphene (TBG), we demonstrate that twisted bilayer boron nitride (TBBN) is an even more exciting novel system that turns out to be an excellent platform to realize new correlated phases and phenomena; exploration of its electronic properties shows that in contrast to TBG in TBBN multiple families of 2,4, and 6-fold degenerate flat bands emerge without the need to fine tune close to a “magic angle”, resulting in dramatic and tunable changes in optical properties and exciton physics, and providing an additional platform to study strong correlations. Upon doping, unforeseen new correlated phases of matter (insulating and superconducting) emerge. TBBN could thus provide a promising experimental platform, insensitive to small deviations in the twist angle, to study novel exciton condensate and spatial confinement physics, and correlations in two dimensions.

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          Most cited references27

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          Principles and applications of electrochemical capacitors

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            Direct-bandgap properties and evidence for ultraviolet lasing of hexagonal boron nitride single crystal.

            The demand for compact ultraviolet laser devices is increasing, as they are essential in applications such as optical storage, photocatalysis, sterilization, ophthalmic surgery and nanosurgery. Many researchers are devoting considerable effort to finding materials with larger bandgaps than that of GaN. Here we show that hexagonal boron nitride (hBN) is a promising material for such laser devices because it has a direct bandgap in the ultraviolet region. We obtained a pure hBN single crystal under high-pressure and high-temperature conditions, which shows a dominant luminescence peak and a series of s-like exciton absorption bands around 215 nm, proving it to be a direct-bandgap material. Evidence for room-temperature ultraviolet lasing at 215 nm by accelerated electron excitation is provided by the enhancement and narrowing of the longitudinal mode, threshold behaviour of the excitation current dependence of the emission intensity, and a far-field pattern of the transverse mode.
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              Atomic and electronic reconstruction at the van der Waals interface in twisted bilayer graphene

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                Author and article information

                Journal
                Nano Lett
                Nano Lett
                nl
                nalefd
                Nano Letters
                American Chemical Society
                1530-6984
                1530-6992
                01 July 2019
                14 August 2019
                : 19
                : 8
                : 4934-4940
                Affiliations
                []Max Planck Institute for the Structure and Dynamics of Matter , Luruper Chaussee 149, 22761 Hamburg, Germany
                []Dahlem Center for Complex Quantum Systems and Fachbereich Physik, Freie Universität Berlin , 14195 Berlin, Germany
                [§ ]Nano-Bio Spectroscopy Group and ETSF, Universidad del País Vasco UPV/EHU , Avenida de Tolosa 72, E-20018 Donostia, Spain
                []Center for Computational Quantum Physics (CCQ), The Flatiron Institute , 162 Fifth Avenue, New York, New York 10010, United States
                Author notes
                Article
                10.1021/acs.nanolett.9b00986
                6699729
                31260633
                550ac963-6df5-4b59-89d6-0fec10c2d643
                Copyright © 2019 American Chemical Society

                This is an open access article published under a Creative Commons Attribution (CC-BY) License, which permits unrestricted use, distribution and reproduction in any medium, provided the author and source are cited.

                History
                : 08 March 2019
                : 22 June 2019
                Categories
                Letter
                Custom metadata
                nl9b00986
                nl-2019-00986r

                Nanotechnology
                twisted bilayer,multiflat bands,strong correlations,mott insulator,topological superconductor,ab initio calculation

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