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      Design and Characterization of Host Frameworks for Facile Magnesium Transport

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          Abstract

          The development of inexpensive batteries based on magnesium (Mg) chemistry will contribute remarkably toward developing high-energy-density storage systems that can be used worldwide. Significant challenges remain in developing practical Mg batteries, the chief of which is designing materials that can provide facile transport of Mg. In this review, we cover the experimental and theoretical methods that can be used to quantify Mg mobility in a variety of host frameworks, the specific transport quantities that each technique is designed to measure or calculate, and some practical examples of their applications. We then list the unique challenges faced by different experimental and computational techniques in probing Mg ion transport in materials. This review concludes with an outlook on the directions that the scientific community could soon pursue as we strive to construct a pragmatic Mg battery.

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            Commentary: The Materials Project: A materials genome approach to accelerating materials innovation

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              A high-capacity and long-life aqueous rechargeable zinc battery using a metal oxide intercalation cathode

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                Author and article information

                Journal
                Annual Review of Materials Research
                Annu. Rev. Mater. Res.
                Annual Reviews
                1531-7331
                1545-4118
                July 01 2022
                July 01 2022
                : 52
                : 1
                : 129-158
                Affiliations
                [1 ]University of Michigan–Shanghai Jiao Tong University Joint Institute, Shanghai Jiao Tong University, Shanghai, China;
                [2 ]Department of Materials Science and Engineering, National University of Singapore, Singapore;
                [3 ]Singapore-MIT Alliance for Research and Technology, Singapore
                [4 ]School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai, China
                [5 ]Department of Materials Engineering, Indian Institute of Science, Bangalore, India;
                [6 ]Department of Chemical and Biomolecular Engineering, National University of Singapore, Singapore
                Article
                10.1146/annurev-matsci-081420-041617
                757d732f-1788-460f-90de-d683e2c5e70e
                © 2022
                History

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