Pressure-induced commensurate order in \({\mathrm{TbMn}}_{2}{\mathrm{O}}_{5}\) and \({\mathrm{DyMn}}_{2}{\mathrm{O}}_{5}\) : Influence of rare-earth anisotropy and $ \mathit{3}\mathit{d}\mathit{\text{−}}\mathit{4}\mathit{f}$ exchange

Magnetism and ferroelectricity are essential to many forms of current technology, and the quest for multiferroic materials, where these two phenomena are intimately coupled, is of great technological and fundamental importance. Ferroelectricity and magnetism tend to be mutually exclusive and interact weakly with each other when they coexist. The exciting new development is the discovery that even a weak magnetoelectric interaction can lead to spectacular cross-coupling effects when it induces electric polarization in a magnetically ordered state. Such magnetic ferroelectricity, showing an unprecedented sensitivity to ap plied magnetic fields, occurs in 'frustrated magnets' with competing interactions between spins and complex magnetic orders. We summarize key experimental findings and the current theoretical understanding of these phenomena, which have great potential for tuneable multifunctional devices.

A new microscopic mechanism of the magneto-electric (ME) effect based on the spin supercurrent is theoretically presented for non-collinear magnets. The close analogy between the superconductors (charge current) and magnets (spin current) is drawn to derive the distribution of the spin supercurrent and the resultant electric polarization. Application to the spiral spin structure is discussed.