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      Catalytic Microtubular Jet Engines Self-Propelled by Accumulated Gas Bubbles

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      Wiley

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          Abstract

          Strain-engineered microtubes with an inner catalytic surface serve as self-propelled microjet engines with speeds of up to approximately 2 mm s(-1) (approximately 50 body lengths per second). The motion of the microjets is caused by gas bubbles ejecting from one opening of the tube, and the velocity can be well approximated by the product of the bubble radius and the bubble ejection frequency. Trajectories of various different geometries are well visualized by long microbubble tails. If a magnetic layer is integrated into the wall of the microjet engine, we can control and localize the trajectories by applying external rotating magnetic fields. Fluid (i.e., fuel) pumping through the microtubes is revealed and directly clarifies the working principle of the catalytic microjet engines.

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          Most cited references28

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          Droplet microfluidics.

          Droplet-based microfluidic systems have been shown to be compatible with many chemical and biological reagents and capable of performing a variety of "digital fluidic" operations that can be rendered programmable and reconfigurable. This platform has dimensional scaling benefits that have enabled controlled and rapid mixing of fluids in the droplet reactors, resulting in decreased reaction times. This, coupled with the precise generation and repeatability of droplet operations, has made the droplet-based microfluidic system a potent high throughput platform for biomedical research and applications. In addition to being used as microreactors ranging from the nano- to femtoliter range; droplet-based systems have also been used to directly synthesize particles and encapsulate many biological entities for biomedicine and biotechnology applications. This review will focus on the various droplet operations, as well as the numerous applications of the system. Due to advantages unique to droplet-based systems, this technology has the potential to provide novel solutions to today's biomedical engineering challenges for advanced diagnostics and therapeutics.
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            Synthetic molecular motors and mechanical machines.

            The widespread use of controlled molecular-level motion in key natural processes suggests that great rewards could come from bridging the gap between the present generation of synthetic molecular systems, which by and large rely upon electronic and chemical effects to carry out their functions, and the machines of the macroscopic world, which utilize the synchronized movements of smaller parts to perform specific tasks. This is a scientific area of great contemporary interest and extraordinary recent growth, yet the notion of molecular-level machines dates back to a time when the ideas surrounding the statistical nature of matter and the laws of thermodynamics were first being formulated. Here we outline the exciting successes in taming molecular-level movement thus far, the underlying principles that all experimental designs must follow, and the early progress made towards utilizing synthetic molecular structures to perform tasks using mechanical motion. We also highlight some of the issues and challenges that still need to be overcome.
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              Self-motile colloidal particles: from directed propulsion to random walk.

              The motion of an artificial microscale swimmer that uses a chemical reaction catalyzed on its own surface to achieve autonomous propulsion is fully characterized experimentally. It is shown that at short times it has a substantial component of directed motion, with a velocity that depends on the concentration of fuel molecules. At longer times, the motion reverts to a random walk with a substantially enhanced diffusion coefficient. Our results suggest strategies for designing artificial chemotactic systems.
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                Author and article information

                Journal
                SMLL
                Small
                Small
                Wiley
                16136810
                16136829
                July 17 2009
                July 17 2009
                : 5
                : 14
                : 1688-1692
                Article
                10.1002/smll.200900021
                19373828
                7eac1e78-78f7-4464-9ee8-96ee49bf93af
                © 2009

                http://doi.wiley.com/10.1002/tdm_license_1.1

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