The New Horizons spacecraft mapped colors and infrared spectra across the encounter hemispheres of Pluto and Charon. The volatile ices CH\(_4\), CO, and N\(_2\), that dominate Pluto's surface, have complicated spatial distributions resulting from sublimation, condensation, and glacial flow acting over seasonal and geological timescales. Pluto's H\(_2\)O ice "bedrock" is also mapped, with isolated outcrops occurring in a variety of settings. Pluto's surface exhibits complex regional color diversity associated with its distinct provinces. Charon's color pattern is simpler, dominated by neutral low latitudes and a reddish northern polar region. Charon near infrared spectra reveal highly localized areas with strong NH\(_3\) absorption tied to small craters with relatively fresh-appearing impact ejecta.