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      Ambient Chemical Fixation of CO 2 Using a Robust Ag 27 Cluster‐Based Two‐Dimensional Metal–Organic Framework

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          Most cited references93

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          Transformation of carbon dioxide.

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            Recent advances in catalytic hydrogenation of carbon dioxide.

            Owing to the increasing emissions of carbon dioxide (CO(2)), human life and the ecological environment have been affected by global warming and climate changes. To mitigate the concentration of CO(2) in the atmosphere various strategies have been implemented such as separation, storage, and utilization of CO(2). Although it has been explored for many years, hydrogenation reaction, an important representative among chemical conversions of CO(2), offers challenging opportunities for sustainable development in energy and the environment. Indeed, the hydrogenation of CO(2) not only reduces the increasing CO(2) buildup but also produces fuels and chemicals. In this critical review we discuss recent developments in this area, with emphases on catalytic reactivity, reactor innovation, and reaction mechanism. We also provide an overview regarding the challenges and opportunities for future research in the field (319 references).
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              Metal-organic framework materials as catalysts.

              A critical review of the emerging field of MOF-based catalysis is presented. Discussed are examples of: (a) opportunistic catalysis with metal nodes, (b) designed catalysis with framework nodes, (c) catalysis by homogeneous catalysts incorporated as framework struts, (d) catalysis by MOF-encapsulated molecular species, (e) catalysis by metal-free organic struts or cavity modifiers, and (f) catalysis by MOF-encapsulated clusters (66 references).
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                Author and article information

                Contributors
                Journal
                Angewandte Chemie International Edition
                Angew. Chem. Int. Ed.
                Wiley
                1433-7851
                1521-3773
                November 02 2020
                August 31 2020
                November 02 2020
                : 59
                : 45
                : 20031-20036
                Affiliations
                [1 ]School of Chemistry and Chemical Engineering Key Lab of Colloid and Interface Chemistry of Ministry of Education State Key Laboratory of Crystal Materials Shandong University Jinan 250100 P. R. China
                [2 ]School of Physics Shandong University Jinan 250100 P. R. China
                [3 ]School of Chemistry and Chemical Engineering Shandong Provincial Key Laboratory of Chemical Energy Storage and Novel Cell Technology Liaocheng University Liaocheng 252000 P. R. China
                [4 ]School of Materials Science and Engineering Shandong University Jinan 250061 P. R. China
                [5 ]Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education) Nankai University Tianjin 300071 China
                [6 ]College of Chemistry Chemical Engineering and Materials Science Shandong Provincial Key Laboratory of Clean Production of Fine Chemicals Shandong Normal University Jinan 250014 P. R. China
                Article
                10.1002/anie.202007122
                8d974e16-0f70-4d58-8ed5-c43e0d3bf0fa
                © 2020

                http://onlinelibrary.wiley.com/termsAndConditions#vor

                http://doi.wiley.com/10.1002/tdm_license_1.1

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