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      Realising high aspect ratio 10 nm feature size in laser materials processing in air at 800 nm wavelength in the far-field by creating a high purity longitudinal light field at focus

      research-article
      , ,
      Light, Science & Applications
      Nature Publishing Group UK
      Optical physics, Laser material processing

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          Abstract

          In semiconductor and data storage device manufacturing, it is desirable to produce feature sizes less than 30 nm with a high depth-to-width aspect ratio on the target material rapidly at a low cost. However, optical diffraction limits the smallest focused laser beam diameter to around half of the laser wavelength ( λ/2). The existing approach to achieving nanoscale fabrication is mainly based on costly extreme ultraviolet (EUV) technology operating within the diffraction limit. In this paper, a new method is shown to achieve materials processing resolution down to 10 nm ( λ/80) at an infrared laser wavelength of around 800 nm in the far-field, in air, well beyond the optical diffraction limit. A high-quality longitudinal field with a purity of 94.7% is generated to realise this super-resolution. Both experiments and theoretical modelling have been carried out to verify and understand the findings. The ablation craters induced on polished silicon, copper, and sapphire are compared for different types of light fields. Holes of 10–30 nm in diameter are produced on sapphire with a depth-to-width aspect ratio of over 16 and a zero taper with a single pulse at 100–120 nJ pulse energy. Such high aspect ratio sub-50 nm holes produced with single pulse laser irradiation are rarely seen in laser processing, indicating a new material removal mechanism with the longitudinal field. The working distance (lens to target) is around 170 µm, thus the material processing is in the far field. Tapered nano-holes can also be produced by adjusting the lens to the target distance.

          Abstract

          Holes of 10–30 nm in diameter are produced on sapphire with a depth to width aspect ratio of over 16 and a zero taper with a single pulse longitudinal field.

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          Most cited references46

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          Metalenses at visible wavelengths: Diffraction-limited focusing and subwavelength resolution imaging.

          Subwavelength resolution imaging requires high numerical aperture (NA) lenses, which are bulky and expensive. Metasurfaces allow the miniaturization of conventional refractive optics into planar structures. We show that high-aspect-ratio titanium dioxide metasurfaces can be fabricated and designed as metalenses with NA = 0.8. Diffraction-limited focusing is demonstrated at wavelengths of 405, 532, and 660 nm with corresponding efficiencies of 86, 73, and 66%. The metalenses can resolve nanoscale features separated by subwavelength distances and provide magnification as high as 170×, with image qualities comparable to a state-of-the-art commercial objective. Our results firmly establish that metalenses can have widespread applications in laser-based microscopy, imaging, and spectroscopy.
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            Cylindrical vector beams: from mathematical concepts to applications

            Qiwen Zhan (2009)
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              Metalenses: Versatile multifunctional photonic components

              Recent progress in metasurface designs fueled by advanced-fabrication techniques has led to the realization of ultrathin, lightweight, and flat lenses (metalenses) with unprecedented functionalities. Due to straightforward fabrication, generally requiring a single-step lithography, and possibility of vertical integration, these planar lenses can potentially replace or complement their conventional refractive and diffractive counterparts leading to further miniaturization of high performance optical devices and systems. Here, we give a brief overview of the evolution of metalenses with an emphasis on the visible and near-infrared spectrum and summarize their important features: diffraction-limited focusing, high quality imaging and multifunctionalities. Future challenges including aberrations’ corrections, as well as current issues and solutions are discussed. We conclude by providing an outlook of this technology platform and by identifying future promising directions.

                Author and article information

                Contributors
                olivier.allegre@manchester.ac.uk
                lin.li@manchester.ac.uk
                Journal
                Light Sci Appl
                Light Sci Appl
                Light, Science & Applications
                Nature Publishing Group UK (London )
                2095-5545
                2047-7538
                2 December 2022
                2 December 2022
                2022
                : 11
                : 339
                Affiliations
                GRID grid.5379.8, ISNI 0000000121662407, Department of Mechanical, Aerospace and Civil Engineering, , The University of Manchester, ; Manchester, M13 9PL UK
                Author information
                http://orcid.org/0000-0003-2627-2517
                Article
                962
                10.1038/s41377-022-00962-x
                9715648
                36456549
                8e9fec9b-bfc1-4336-8cfe-ae72cf637636
                © The Author(s) 2022

                Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.

                History
                : 8 December 2021
                : 5 July 2022
                : 18 August 2022
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                © The Author(s) 2022

                optical physics,laser material processing
                optical physics, laser material processing

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