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      Aerial strategies advance volcanic gas measurements at inaccessible, strongly degassing volcanoes

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          Abstract

          Aerial measurements using unoccupied aerial systems (UAS) transform our ability to measure and monitor volcanic plumes.

          Abstract

          Volcanic emissions are a critical pathway in Earth’s carbon cycle. Here, we show that aerial measurements of volcanic gases using unoccupied aerial systems (UAS) transform our ability to measure and monitor plumes remotely and to constrain global volatile fluxes from volcanoes. Combining multi-scale measurements from ground-based remote sensing, long-range aerial sampling, and satellites, we present comprehensive gas fluxes—3760 ± [600, 310] tons day −1 CO 2 and 5150 ± [730, 340] tons day −1 SO 2—for a strong yet previously uncharacterized volcanic emitter: Manam, Papua New Guinea. The CO 2/S T ratio of 1.07 ± 0.06 suggests a modest slab sediment contribution to the sub-arc mantle. We find that aerial strategies reduce uncertainties associated with ground-based remote sensing of SO 2 flux and enable near–real-time measurements of plume chemistry and carbon isotope composition. Our data emphasize the need to account for time averaging of temporal variability in volcanic gas emissions in global flux estimates.

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          Most cited references103

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          New Equations for Computing Vapor Pressure and Enhancement Factor

          Arden Buck (1981)
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            Origin of carbon in fumarolic gas from island arcs

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              Magmatic gas composition reveals the source depth of slug-driven strombolian explosive activity.

              Strombolian-type eruptive activity, common at many volcanoes, consists of regular explosions driven by the bursting of gas slugs that rise faster than surrounding magma. Explosion quakes associated with this activity are usually localized at shallow depth; however, where and how slugs actually form remain poorly constrained. We used spectroscopic measurements performed during both quiescent degassing and explosions on Stromboli volcano (Italy) to demonstrate that gas slugs originate from as deep as the volcano-crust interface (approximately 3 kilometers), where both structural discontinuities and differential bubble-rise speed can promote slug coalescence. The observed decoupling between deep slug genesis and shallow (approximately 250-meter) explosion quakes may be a common feature of strombolian activity, determined by the geometry of plumbing systems.
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                Author and article information

                Journal
                Sci Adv
                Sci Adv
                SciAdv
                advances
                Science Advances
                American Association for the Advancement of Science
                2375-2548
                October 2020
                30 October 2020
                : 6
                : 44
                : eabb9103
                Affiliations
                [1 ]University College London, London WC1E6BS, UK.
                [2 ]University of Cambridge, Cambridge CB23EQ, UK.
                [3 ]Università di Palermo, 90123 Palermo, Italy.
                [4 ]GasLAB, Universidad de Costa Rica, San José, Costa Rica.
                [5 ]Chalmers University of Technology, Göteborg, Sweden.
                [6 ]Heidelberg University, Heidelberg, Germany.
                [7 ]Max Planck Institute for Chemistry, Mainz, Germany.
                [8 ]Michigan Technological University, Houghton, MI 49931, USA.
                [9 ]University of Bristol, Bristol, BS8 1TR, UK.
                [10 ]Universidad Nacional, Heredia, 40101-3000 Costa Rica.
                [11 ]University of New Mexico, Albuquerque, NM 87131, USA.
                [12 ]University of Saskatchewan, Centre for Hydrology, Canmore, Alberta T1W 3G1, Canada.
                [13 ]INGV, Osservatorio Etneo, Sezione di Catania, 95125 Catania, Italy.
                [14 ]Johannes Gutenberg-Universität, Mainz 55128, Germany.
                [15 ]University of Manchester, Manchester, M13 9PL, UK.
                [16 ]Rabaul Volcanological Observatory, Rabaul, Papua New Guinea.
                [17 ]Victoria University of Wellington, Wellington 6012, New Zealand.
                Author notes
                [* ]Corresponding author. Email: emma.liu@ 123456ucl.ac.uk
                Author information
                http://orcid.org/0000-0003-1749-9285
                http://orcid.org/0000-0002-0254-6539
                http://orcid.org/0000-0002-6975-7066
                http://orcid.org/0000-0002-0306-3782
                http://orcid.org/0000-0003-0460-9772
                http://orcid.org/0000-0002-0360-6660
                http://orcid.org/0000-0002-5485-2992
                http://orcid.org/0000-0002-0494-3466
                http://orcid.org/0000-0003-2380-5832
                http://orcid.org/0000-0002-9628-3329
                http://orcid.org/0000-0003-1243-137X
                http://orcid.org/0000-0002-3467-0649
                http://orcid.org/0000-0002-4466-8649
                http://orcid.org/0000-0001-9989-809X
                http://orcid.org/0000-0002-2534-8041
                http://orcid.org/0000-0002-9410-4139
                http://orcid.org/0000-0002-2188-5384
                http://orcid.org/0000-0001-5734-0549
                http://orcid.org/0000-0001-9877-2065
                http://orcid.org/0000-0002-7050-6475
                http://orcid.org/0000-0002-3025-9190
                http://orcid.org/0000-0003-1524-4262
                http://orcid.org/0000-0001-7767-452X
                http://orcid.org/0000-0001-9198-2203
                http://orcid.org/0000-0002-5804-7704
                Article
                abb9103
                10.1126/sciadv.abb9103
                7608812
                33127674
                90843248-43a3-493e-945c-429542c7d85b
                Copyright © 2020 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution License 4.0 (CC BY).

                This is an open-access article distributed under the terms of the Creative Commons Attribution license, which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.

                History
                : 06 April 2020
                : 18 September 2020
                Funding
                Funded by: doi http://dx.doi.org/10.13039/100000001, National Science Foundation;
                Award ID: EAR-1664246
                Funded by: doi http://dx.doi.org/10.13039/100000879, Alfred P. Sloan Foundation;
                Funded by: doi http://dx.doi.org/10.13039/501100000275, Leverhulme Trust;
                Funded by: doi http://dx.doi.org/10.13039/501100001509, Royal Society of New Zealand;
                Award ID: 18-VUW-023
                Funded by: doi http://dx.doi.org/10.13039/501100001859, Swedish National Space Board;
                Funded by: doi http://dx.doi.org/10.13039/501100001862, Swedish Research Council Formas;
                Funded by: Ministero Istruzione Università e Ricerca of Italy;
                Award ID: PRIN2017-2017LMNLAW
                Funded by: doi http://dx.doi.org/10.13039/501100007601, Horizon 2020;
                Award ID: EUROVOLC
                Categories
                Research Article
                Research Articles
                SciAdv r-articles
                Physical Sciences
                Applied Sciences and Engineering
                Custom metadata
                Kyle Solis

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