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      Dynamics of wrinkling in ultrathin elastic sheets

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          Significance

          Elastic instabilities provide a means of generating regular topographies with a well-defined wavelength. For example, a thin elastic film attached to a softer substrate buckles into an array of regular wrinkles under quasistatic compression. The wrinkle wavelength is selected by the mechanical properties of the system so that different wavelengths are typically attained through variation of the film thickness. Here, we show that, for a film of given thickness, variation in the wrinkle wavelength can be achieved dynamically. Our study of impact-induced wrinkling demonstrates that the inertial response of the substrate results in an evolving wrinkle wavelength, opening the route toward dynamic tuning of wrinkle-patterned topographies.

          Abstract

          The wrinkling of thin elastic objects provides a means of generating regular patterning at small scales in applications ranging from photovoltaics to microfluidic devices. Static wrinkle patterns are known to be governed by an energetic balance between the object’s bending stiffness and an effective substrate stiffness, which may originate from a true substrate stiffness or from tension and curvature along the wrinkles. Here, we investigate dynamic wrinkling induced by the impact of a solid sphere onto an ultrathin polymer sheet floating on water. The vertical deflection of the sheet’s center induced by impact draws material radially inward, resulting in an azimuthal compression that is relieved by the wrinkling of the entire sheet. We show that this wrinkling is truly dynamic, exhibiting features that are qualitatively different to those seen in quasistatic wrinkling experiments. Moreover, we show that the wrinkles coarsen dynamically because of the inhibiting effect of the fluid inertia. This dynamic coarsening can be understood heuristically as the result of a dynamic stiffness, which dominates the static stiffnesses reported thus far, and allows control of wrinkle wavelength.

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          Most cited references42

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          A buckling-based metrology for measuring the elastic moduli of polymeric thin films.

          As technology continues towards smaller, thinner and lighter devices, more stringent demands are placed on thin polymer films as diffusion barriers, dielectric coatings, electronic packaging and so on. Therefore, there is a growing need for testing platforms to rapidly determine the mechanical properties of thin polymer films and coatings. We introduce here an elegant, efficient measurement method that yields the elastic moduli of nanoscale polymer films in a rapid and quantitative manner without the need for expensive equipment or material-specific modelling. The technique exploits a buckling instability that occurs in bilayers consisting of a stiff, thin film coated onto a relatively soft, thick substrate. Using the spacing of these highly periodic wrinkles, we calculate the film's elastic modulus by applying well-established buckling mechanics. We successfully apply this new measurement platform to several systems displaying a wide range of thicknessess (nanometre to micrometre) and moduli (MPa to GPa).
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            Capillary wrinkling of floating thin polymer films.

            A freely floating polymer film, tens of nanometers in thickness, wrinkles under the capillary force exerted by a drop of water placed on its surface. The wrinkling pattern is characterized by the number and length of the wrinkles. The dependence of the number of wrinkles on the elastic properties of the film and on the capillary force exerted by the drop confirms recent theoretical predictions on the selection of a pattern with a well-defined length scale in the wrinkling instability. We combined scaling relations that were developed for the length of the wrinkles with those for the number of wrinkles to construct a metrology for measuring the elasticity and thickness of ultrathin films that relies on no more than a dish of fluid and a low-magnification microscope. We validated this method on polymer films modified by plasticizer. The relaxation of the wrinkles affords a simple method to study the viscoelastic response of ultrathin films.
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              Harnessing Surface Wrinkle Patterns in Soft Matter

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                Author and article information

                Journal
                Proc Natl Acad Sci U S A
                Proc. Natl. Acad. Sci. U.S.A
                pnas
                pnas
                PNAS
                Proceedings of the National Academy of Sciences of the United States of America
                National Academy of Sciences
                0027-8424
                1091-6490
                15 October 2019
                30 September 2019
                30 September 2019
                : 116
                : 42
                : 20875-20880
                Affiliations
                [1] aMathematical Institute, University of Oxford, Oxford OX2 6GG, United Kingdom;
                [2] bDepartment of Engineering Science, University of Oxford, Oxford OX1 3PJ, United Kingdom
                Author notes
                1To whom correspondence may be addressed. Email: dominic.vella@ 123456maths.ox.ac.uk .

                Edited by Howard A. Stone, Princeton University, Princeton, NJ, and approved August 29, 2019 (received for review April 12, 2019)

                Author contributions: D.V. designed research; F.B., D.O’K., O.K., M.I., A.A.C.-P., and D.V. performed research; F.B. and D.O’K. analyzed data; and F.B., D.O’K., and D.V. wrote the paper.

                Author information
                http://orcid.org/0000-0003-1341-8863
                Article
                201905755
                10.1073/pnas.1905755116
                6800320
                31570627
                93a7212e-a71e-4a39-8d92-fa802ae57c78
                Copyright © 2019 the Author(s). Published by PNAS.

                This open access article is distributed under Creative Commons Attribution-NonCommercial-NoDerivatives License 4.0 (CC BY-NC-ND).

                History
                Page count
                Pages: 6
                Funding
                Funded by: European Research Council
                Award ID: 637334
                Award Recipient : Dominic Vella
                Categories
                Physical Sciences
                Physics
                From the Cover

                dynamic wrinkling,impact,elastocapillarity,fluid–structure interaction

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