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      Highly enantioselective S–H bond insertion cooperatively catalyzed by dirhodium complexes and chiral spiro phosphoric acids

      , , , , ,
      Chemical Science
      Royal Society of Chemistry (RSC)

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          Transition-metal-catalyzed C-S, C-Se, and C-Te bond formation via cross-coupling and atom-economic addition reactions.

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            Metal-Catalyzed Carbon−Sulfur Bond Formation

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              Unifying metal and Brønsted acid catalysis--concepts, mechanisms, and classifications.

              Asymmetric catalysis is a key feature of modern synthetic organic chemistry. Traditionally, different combinations of ligands and metals are used to perform highly enantioselective reactions. Since the renaissance of organocatalysis in the early 2000s, tremendous improvement in the field of metal-free catalysis has been achieved. Recently, the combination of transition metals and organocatalysts has allowed the development of new protocols enabling transformations that could not previously be realized. This article aims to present the latest contributions in the field of combined chiral Brønsted acid and metal catalyzed reactions, highlighting the advantages of these catalytic systems as well as describing the uncertainties regarding the molecular structure of the catalytically active species and the reaction mechanisms.
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                Author and article information

                Journal
                CSHCBM
                Chemical Science
                Chem. Sci.
                Royal Society of Chemistry (RSC)
                2041-6520
                2041-6539
                2014
                2014
                : 5
                : 4
                : 1442
                Article
                10.1039/c3sc52807c
                a0b548e5-4d91-410d-8f5e-5be19ea23669
                © 2014
                History

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