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      Single-Atom Pt as Co-Catalyst for Enhanced Photocatalytic H2 Evolution.

      Advanced Materials (Deerfield Beach, Fla.)
      Wiley
      photocatalysis, single-atom co-catalysts, H2 evolution, atom efficiency, graphitic carbon nitride

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          Abstract

          Isolated single-atom platinum (Pt) embedded in the sub-nanoporosity of 2D g-C3 N4 as a new form of co-catalyst is reported. The highly stable single-atom co-catalyst maximizes the atom efficiency and alters the surface trap states of g-C3 N4 , leading to significantly enhanced photocatalytic H2 evolution activity, 8.6 times higher than that of Pt nanoparticles and up to 50 times that for bare g-C3 N4 .

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          Author and article information

          Journal
          26822495
          10.1002/adma.201505281

          photocatalysis,single-atom co-catalysts,H2 evolution,atom efficiency,graphitic carbon nitride

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