Total Synthesis of Transtaganolide E and F: Insight in the Biosynthesis of the Transtaganolides

Aben, Rene W. M.; Sterner, Olov; Scheeren, Hans W; Larsson, Rikard; Johansson, Martin

doi:10.1002/ejoc.201301092

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Total Synthesis of Transtaganolide E and F: Insight in the Biosynthesis of the Transtaganolides : Total Synthesis of Transtaganolide E and F

Author(s): Rikard Larsson , Hans W. Scheeren , Rene W. M. Aben , Martin Johansson , Olov Sterner

Publication date Created: October 2013

Publication date (Print): October 11 2013

Journal: European Journal of Organic Chemistry

Publisher: Wiley-Blackwell

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Progress toward the Synthesis of the Basiliolides and Transtaganolides: An Intramolecular Pyrone Diels−Alder Entry into a Novel Class of Natural Products

Brian Stoltz, Hosea M. Nelson (2008)

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A pyran-2-one and four meroterpenoids from Thapsia transtagana and their implication in the biosynthesis of transtaganolides.

F Guerra, Abderrahmane Saouf, Guillermo Massanet … (2007)

Four meroterpenoids (3a, 3b, 4 and 5), a prenylated pyran-2-one (2) along with the known compounds 7-O-geranylscopoletin (1), and thapsitranstagin (6) have been isolated from the roots of Thapsia transtagana. The presence of 1 and 2 supports the biogenetic hypothesis that transtaganolides, a group of bioactive metabolites, are meroterpenoids which come from an O-prenylated coumarin via successive pericyclic reactions.