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      Efficient generation of ortho-quinone methide: application to the biomimetic syntheses of (±)-schefflone and tocopherol trimers.

      1 , ,
      Organic letters

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          Abstract

          An efficient method using silver oxide-mediated oxidation for the synthesis of ortho-quinone methides has been developed and applied to the biomimetic syntheses of novel trimeric natural products, (±)-schefflone and tocopherol trimers. Further studies of the critical trimerization as well as substrate scope and limitations are also reported.

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          Author and article information

          Journal
          Org. Lett.
          Organic letters
          1523-7052
          1523-7052
          Jan 6 2012
          : 14
          : 1
          Affiliations
          [1 ] School of Pharmaceutical Science and Technology, Tianjin University, Tianjin 300072, China.
          Article
          10.1021/ol202641y
          22047096
          b5c4d6cb-941b-4b66-9599-cadf34b7aa39
          © 2011 American Chemical Society
          History

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