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      Silicon clusters produced by femtosecond laser ablation: Non-thermal emission and gas-phase condensation

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          Abstract

          Neutral silicon clusters Si_n (up to n = 7) and their cations Si_n+ (up to n = 10) have been produced by femtosecond laser ablation of bulk silicon in vacuum and investigated using time-of-flight mass spectrometry. Two populations of the Si_n+ clusters with different velocity and abundance distributions in the ablation plume have been clearly distinguished. Possible mechanisms of cluster formation (Coulomb explosion, gas-phase condensation, phase explosion) are discussed.

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          Author and article information

          Journal
          10 March 2004
          Article
          10.1007/s00339-004-2856-y
          physics/0403060
          d905e29d-1fcf-45ba-ba64-a5a36e88df41
          History
          Custom metadata
          Applied Physics A 79 (2004) 1591-1594
          physics.atm-clus physics.chem-ph physics.plasm-ph
          ccsd ccsd-00001265

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