Engineering of Fermi level by nin diamond junction for control of charge states of NV centers

Projective measurement of single electron and nuclear spins has evolved from a gedanken experiment to a problem relevant for applications in atomic-scale technologies like quantum computing. Although several approaches allow for detection of a spin of single atoms and molecules, multiple repetitions of the experiment that are usually required for achieving a detectable signal obscure the intrinsic quantum nature of the spin's behavior. We demonstrated single-shot, projective measurement of a single nuclear spin in diamond using a quantum nondemolition measurement scheme, which allows real-time observation of an individual nuclear spin's state in a room-temperature solid. Such an ideal measurement is crucial for realization of, for example, quantum error correction protocols in a quantum register.

Robust entanglement at room temperature is a necessary requirement for practical applications in quantum technology. We demonstrate the creation of bipartite- and tripartite-entangled quantum states in a small quantum register consisting of individual 13C nuclei in a diamond lattice. Individual nuclear spins are controlled via their hyperfine coupling to a single electron at a nitrogen-vacancy defect center. Quantum correlations are of high quality and persist on a millisecond time scale even at room temperature, which is adequate for sophisticated quantum operations.

Quantum entanglement between spatially separated objects is one of the most intriguing phenomena in physics. The outcomes of independent measurements on entangled objects show correlations that cannot be explained by classical physics. Besides being of fundamental interest, entanglement is a unique resource for quantum information processing and communication. Entangled qubits can be used to establish private information or implement quantum logical gates. Such capabilities are particularly useful when the entangled qubits are spatially separated, opening the opportunity to create highly connected quantum networks or extend quantum cryptography to long distances. Here we present a key experiment towards the realization of long-distance quantum networks with solid-state quantum registers. We have entangled two electron spin qubits in diamond that are separated by a three-meter distance. We establish this entanglement using a robust protocol based on local creation of spin-photon entanglement and a subsequent joint measurement of the photons. Detection of the photons heralds the projection of the spin qubits onto an entangled state. We verify the resulting non-local quantum correlations by performing single-shot readout on the qubits in different bases. The long-distance entanglement reported here can be combined with recently achieved initialization, readout and entanglement operations on local long-lived nuclear spin registers, enabling deterministic long-distance teleportation, quantum repeaters and extended quantum networks.