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      Hydroxy-functionalized hyper-cross-linked ultra-microporous organic polymers for selective CO 2 capture at room temperature

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          Summary

          Two hydroxy-functionalized hyper-cross-linked ultra-microporous compounds have been synthesized by Friedel–Crafts alkylation reaction and characterised with different spectroscopic techniques. Both compounds exhibit an efficient carbon dioxide uptake over other gases like N 2, H 2 and O 2 at room temperature. A high isosteric heat of adsorption ( Q st) has been obtained for both materials because of strong interactions between polar –OH groups and CO 2 molecules.

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          Conjugated microporous polymers: design, synthesis and application.

          Yanhong Xu, Shangbin Jin, Hong Xu … (2013)
          Conjugated microporous polymers (CMPs) are a class of organic porous polymers that combine π-conjugated skeletons with permanent nanopores, in sharp contrast to other porous materials that are not π-conjugated and with conventional conjugated polymers that are nonporous. As an emerging material platform, CMPs offer a high flexibility for the molecular design of conjugated skeletons and nanopores. Various chemical reactions, building blocks and synthetic methods have been developed and a broad variety of CMPs with different structures and specific properties have been synthesized, driving the rapid growth of the field. CMPs are unique in that they allow the complementary utilization of π-conjugated skeletons and nanopores for functional exploration; they have shown great potential for challenging energy and environmental issues, as exemplified by their excellent performance in gas adsorption, heterogeneous catalysis, light emitting, light harvesting and electrical energy storage. This review describes the molecular design principles of CMPs, advancements in synthetic and structural studies and the frontiers of functional exploration and potential applications.
          Article 0 comments Cited 393 times – based on 0 reviews     Review now
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            Targeted Synthesis of a Porous Aromatic Framework with High Stability and Exceptionally High Surface Area

            Teng Ben, Hao Ren, Shengqian Ma … (2009)
            Article 0 comments Cited 386 times – based on 0 reviews     Review now
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              Exploitation of Intrinsic Microporosity in Polymer-Based Materials

              Peter Budd, Neil McKeown (2010)
              Article 0 comments Cited 204 times – based on 0 reviews     Review now
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                Author and article information

                Contributors
                Sujit K Ghosh
                Stefan Bräse: Role: Guest Editor
                Journal
                Journal ID (nlm-ta): Beilstein J Org Chem
                Journal ID (iso-abbrev): Beilstein J Org Chem
                Title: Beilstein Journal of Organic Chemistry
                Publisher: Beilstein-Institut (Trakehner Str. 7-9, 60487 Frankfurt am Main, Germany )
                ISSN (Electronic): 1860-5397
                Publication date Collection: 2016
                Publication date (Electronic): 2 September 2016
                Volume: 12
                Pages: 1981-1986
                Affiliations
                [1 ]Indian Institute of Science Education and Research (IISER), Pune. Dr. Homi Bhabha Road, Pashan, Pune-411008, India. Fax: +91 20 2589 8022; Tel: +91 20 2590 8076
                [2 ]Centre for Research in Energy & Sustainable Materials, IISER Pune, Pashan, Pune, India
                Article
                DOI: 10.3762/bjoc.12.185
                PMC ID: 5082474
                PubMed ID: 27829902
                SO-VID: e5de8cd9-11f9-460f-bc3a-dd9f3bdeeff8
                Copyright © Copyright © 2016, Samanta et al.; licensee Beilstein-Institut.
                License:

                This is an Open Access article under the terms of the Creative Commons Attribution License ( http://creativecommons.org/licenses/by/4.0), which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.

                The license is subject to the Beilstein Journal of Organic Chemistry terms and conditions: ( http://www.beilstein-journals.org/bjoc)

                History
                Date received : 9 July 2016
                Date accepted : 19 August 2016
                Categories
                Subject: Letter
                Subject: Chemistry
                Subject: Organic Chemistry

                ScienceOpen disciplines: Organic & Biomolecular chemistry
                Keywords: carbon dioxide capture,hyper-cross-linked polymer,metal-organic framework,microporous organic polymer
                Data availability:
                ScienceOpen disciplines: Organic & Biomolecular chemistry
                Keywords: carbon dioxide capture, hyper-cross-linked polymer, metal-organic framework, microporous organic polymer

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