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Noble metal nanoparticles/carbon nanotubes nanohybrids: Synthesis and applications

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Nano Today

Elsevier BV

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      Helical microtubules of graphitic carbon

       Sumio Iijima (1991)
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        Nitrogen-doped carbon nanotube arrays with high electrocatalytic activity for oxygen reduction.

        The large-scale practical application of fuel cells will be difficult to realize if the expensive platinum-based electrocatalysts for oxygen reduction reactions (ORRs) cannot be replaced by other efficient, low-cost, and stable electrodes. Here, we report that vertically aligned nitrogen-containing carbon nanotubes (VA-NCNTs) can act as a metal-free electrode with a much better electrocatalytic activity, long-term operation stability, and tolerance to crossover effect than platinum for oxygen reduction in alkaline fuel cells. In air-saturated 0.1 molar potassium hydroxide, we observed a steady-state output potential of -80 millivolts and a current density of 4.1 milliamps per square centimeter at -0.22 volts, compared with -85 millivolts and 1.1 milliamps per square centimeter at -0.20 volts for a platinum-carbon electrode. The incorporation of electron-accepting nitrogen atoms in the conjugated nanotube carbon plane appears to impart a relatively high positive charge density on adjacent carbon atoms. This effect, coupled with aligning the NCNTs, provides a four-electron pathway for the ORR on VA-NCNTs with a superb performance.
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          Filamentous growth of carbon through benzene decomposition

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            Author and article information

            Journal
            Nano Today
            Nano Today
            Elsevier BV
            17480132
            February 2011
            February 2011
            : 6
            : 1
            : 75-90
            10.1016/j.nantod.2010.12.008
            © 2011

            http://www.elsevier.com/tdm/userlicense/1.0/

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