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      Bi 1Te 1 is a dual topological insulator

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          Abstract

          New three-dimensional (3D) topological phases can emerge in superlattices containing constituents of known two-dimensional topologies. Here we demonstrate that stoichiometric Bi 1Te 1, which is a natural superlattice of alternating two Bi 2Te 3 quintuple layers and one Bi bilayer, is a dual 3D topological insulator where a weak topological insulator phase and topological crystalline insulator phase appear simultaneously. By density functional theory, we find indices (0;001) and a non-zero mirror Chern number. We have synthesized Bi 1Te 1 by molecular beam epitaxy and found evidence for its topological crystalline and weak topological character by spin- and angle-resolved photoemission spectroscopy. The dual topology opens the possibility to gap the differently protected metallic surface states on different surfaces independently by breaking the respective symmetries, for example, by magnetic field on one surface and by strain on another surface.

          Abstract

          Coexistence of a topological insulator phase and a topological crystalline insulator phase helps to maintain topological properties under a controlled symmetry breaking perturbation. Here, Eschback et al. report a superlattice of Bi and Bi 2Te 3 to be such a dual topological insulator.

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          Most cited references33

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          Generalized Gradient Approximation Made Simple.

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            Topological crystalline insulators.

            Liang Fu (2011)
            The recent discovery of topological insulators has revived interest in the band topology of insulators. In this Letter, we extend the topological classification of band structures to include certain crystal point group symmetry. We find a class of three-dimensional "topological crystalline insulators" which have metallic surface states with quadratic band degeneracy on high symmetry crystal surfaces. These topological crystalline insulators are the counterpart of topological insulators in materials without spin-orbit coupling. Their band structures are characterized by new topological invariants. We hope this work will enlarge the family of topological phases in band insulators and stimulate the search for them in real materials.
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              Observation of unconventional quantum spin textures in topological insulators.

              A topologically ordered material is characterized by a rare quantum organization of electrons that evades the conventional spontaneously broken symmetry-based classification of condensed matter. Exotic spin-transport phenomena, such as the dissipationless quantum spin Hall effect, have been speculated to originate from a topological order whose identification requires a spin-sensitive measurement, which does not exist to this date in any system. Using Mott polarimetry, we probed the spin degrees of freedom and demonstrated that topological quantum numbers are completely determined from spin texture-imaging measurements. Applying this method to Sb and Bi(1-x)Sb(x), we identified the origin of its topological order and unusual chiral properties. These results taken together constitute the first observation of surface electrons collectively carrying a topological quantum Berry's phase and definite spin chirality, which are the key electronic properties component for realizing topological quantum computing bits with intrinsic spin Hall-like topological phenomena.
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                Author and article information

                Journal
                Nat Commun
                Nat Commun
                Nature Communications
                Nature Publishing Group
                2041-1723
                21 April 2017
                2017
                : 8
                : 14976
                Affiliations
                [1 ]Peter Grünberg Institut and JARA-FIT, Forschungszentrum Jülich GmbH , 52425 Jülich, Germany
                [2 ]Institute for Advanced Simulation, Forschungszentrum Jülich GmbH , 52425 Jülich, Germany
                [3 ]Faculty of Physics and Applied Computer Science, AGH University of Science and Technology , al. Mickiewicza 30, Krakow 30-059, Poland
                [4 ]II. Institute of Physics B and JARA-FIT, RWTH Aachen University , Aachen 52074, Germany
                [5 ]Faculty of Physics, University of Duisburg-Essen , D-47057 Duisburg, Germany
                [6 ]Ernst Ruska-Centre for Microscopy and Spectroscopy with Electrons, Forschungszentrum Jülich GmbH , Wilhelm-Johnen-Straße, 52425 Jülich, Germany
                Author notes
                [*]

                These authors contributed equally to this work.

                Author information
                http://orcid.org/0000-0002-5613-7570
                http://orcid.org/0000-0002-6615-1122
                Article
                ncomms14976
                10.1038/ncomms14976
                5413958
                28429708
                f6679d23-c1ae-403a-b5cb-4748f3c1dbad
                Copyright © 2017, The Author(s)

                This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article's Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/

                History
                : 25 May 2016
                : 16 February 2017
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