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      Photoelectron imaging on time-dependent molecular alignment created by a femtosecond laser pulse.

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          Abstract

          Rotational wave packet revivals on an excited electronic state have been measured by femtosecond time-resolved photoelectron imaging for the first time. The first full revival at 82 ps of S1 (n,pi*) pyrazine was clearly observed in the time dependencies of the photoelectron intensity and the photoelectron angular distribution (PAD). The PAD, measured for laser aligned pyrazine, clearly reflects the different characters of pi* and 3s molecular orbitals.

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          Most cited references27

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          Velocity map imaging of ions and electrons using electrostatic lenses: Application in photoelectron and photofragment ion imaging of molecular oxygen

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            On the Angular Distribution in Nuclear Reactions and Coincidence Measurements

            C. N. Yang (1948)
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              Electronic states of azabenzenes and azanaphthalenes: A revised and extended critical review

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                Author and article information

                Journal
                Phys. Rev. Lett.
                Physical review letters
                American Physical Society (APS)
                0031-9007
                0031-9007
                May 14 2001
                : 86
                : 20
                Affiliations
                [1 ] Graduate University for Advanced Studies, Myodaiji, Okazaki 444-8585, Japan.
                Article
                10.1103/PhysRevLett.86.4500
                11384268
                f6746a2c-489e-41e4-a078-f4b89559ed99
                History

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