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      Domino N-/C-Arylation via In Situ Generation of a Directing Group: Atom-Efficient Arylation Using Diaryliodonium Salts.

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          Abstract

          Both aryl components of diaryliodonium salts can be used in a domino one-pot reaction via in situ generation of a directing group. A number of heterocycles undergo N-arylation which is followed by ruthenium-catalyzed C-arylation. Notably the reaction extends well to unsymmetrical diaryliodonium salts with a number of highly selective examples shown.

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          Author and article information

          Journal
          Angew. Chem. Int. Ed. Engl.
          Angewandte Chemie (International ed. in English)
          Wiley-Blackwell
          1521-3773
          1433-7851
          May 02 2017
          : 56
          : 19
          Affiliations
          [1 ] School of Chemistry, The University of Manchester, Oxford Road, Manchester, M13 9PL, UK.
          Article
          10.1002/anie.201701523
          28387054

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