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      Photo-induced cascaded harmonic and comb generation in silicon nitride microresonators

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          Abstract

          Silicon nitride (Si 3N 4) is an ever-maturing integrated platform for nonlinear optics but mostly considered for third-order [χ (3)] nonlinear interactions. Recently, second-order [χ (2)] nonlinearity was introduced into Si 3N 4 via the photogalvanic effect, resulting in the inscription of quasi-phase–matched χ (2) gratings. However, the full potential of the photogalvanic effect in microresonators remains largely unexplored for cascaded effects. Here, we report combined χ (2) and χ (3) nonlinear effects in a normal dispersion Si 3N 4 microresonator. We demonstrate that the photo-induced χ (2) grating also provides phase-matching for the sum-frequency generation process, enabling the initiation and successive switching of primary combs. In addition, the doubly resonant pump and second-harmonic fields allow for effective third-harmonic generation, where a secondary optically written χ (2) grating is identified. Last, we reach a broadband microcomb state evolved from the sum-frequency–coupled primary comb. These results expand the scope of cascaded effects in microresonators.

          Abstract

          Abstract

          Light can induce second order nonlinearity in microrings and can enable frequency conversion and comb generation afterwards.

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          Dissipative Kerr solitons in optical microresonators

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            Temporal solitons in optical microresonators

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              Ultralow-threshold Raman laser using a spherical dielectric microcavity.

              The ability to confine and store optical energy in small volumes has implications in fields ranging from cavity quantum electrodynamics to photonics. Of all cavity geometries, micrometre-sized dielectric spherical resonators are the best in terms of their ability to store energy for long periods of time within small volumes. In the sphere, light orbits near the surface, where long confinement times (high Q) effectively wrap a large interaction distance into a tiny volume. This characteristic makes such resonators uniquely suited for studies of nonlinear coupling of light with matter. Early work recognized these attributes through Raman excitation in microdroplets-but microdroplets have not been used in practical applications. Here we demonstrate a micrometre-scale, nonlinear Raman source that has a highly efficient pump-signal conversion (higher than 35%) and pump thresholds nearly 1,000 times lower than shown before. This represents a route to compact, ultralow-threshold sources for numerous wavelength bands that are usually difficult to access. Equally important, this system can provide a compact and simple building block for studying nonlinear optical effects and the quantum aspects of light.
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                Author and article information

                Contributors
                Role: ConceptualizationRole: Data curationRole: Formal analysisRole: InvestigationRole: MethodologyRole: Project administrationRole: ResourcesRole: SoftwareRole: SupervisionRole: ValidationRole: VisualizationRole: Writing - original draftRole: Writing - review & editing
                Role: ConceptualizationRole: Formal analysisRole: InvestigationRole: MethodologyRole: Project administrationRole: ResourcesRole: SoftwareRole: ValidationRole: VisualizationRole: Writing - original draft
                Role: ConceptualizationRole: InvestigationRole: MethodologyRole: ResourcesRole: ValidationRole: Writing - original draft
                Role: ConceptualizationRole: InvestigationRole: Project administrationRole: ResourcesRole: Writing - review & editing
                Role: ConceptualizationRole: MethodologyRole: Writing - review & editing
                Role: Writing - original draftRole: Writing - review & editing
                Role: ConceptualizationRole: Funding acquisitionRole: MethodologyRole: Project administrationRole: ResourcesRole: SupervisionRole: ValidationRole: VisualizationRole: Writing - original draftRole: Writing - review & editing
                Role: ConceptualizationRole: Funding acquisitionRole: Project administrationRole: SupervisionRole: ValidationRole: Writing - original draftRole: Writing - review & editing
                Journal
                Sci Adv
                Sci Adv
                sciadv
                advances
                Science Advances
                American Association for the Advancement of Science
                2375-2548
                December 2022
                14 December 2022
                : 8
                : 50
                : eadd8252
                Affiliations
                [ 1 ]École Polytechnique Fédérale de Lausanne, Photonic Systems Laboratory (PHOSL), STI-IEM, Station 11, Lausanne CH-1015, Switzerland.
                [ 2 ]École Polytechnique Fédérale de Lausanne, Laboratory of Photonics and Quantum Measurements (LPQM), SB-IPHYS, Station 3, Lausanne CH-1015, Switzerland.
                Author notes
                [†]

                These authors contributed equally to the work.

                [‡]

                Present address: Institute for Photonics and Advanced Sensing (IPAS) and School of Physical Sciences, The University of Adelaide, Adelaide, South Australia 5005, Australia.

                [* ]Corresponding author. Email: camille.bres@ 123456epfl.ch
                Author information
                https://orcid.org/0000-0002-2018-253X
                https://orcid.org/0000-0001-7011-4386
                https://orcid.org/0000-0003-2405-6028
                https://orcid.org/0000-0003-2628-5174
                https://orcid.org/0000-0002-3408-886X
                https://orcid.org/0000-0003-2804-1675
                Article
                add8252
                10.1126/sciadv.add8252
                9750138
                36516262
                534a9a65-2227-4ff8-b43b-435691863b66
                Copyright © 2022 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC).

                This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license, which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited.

                History
                : 06 July 2022
                : 08 November 2022
                Funding
                Funded by: FundRef http://dx.doi.org/10.13039/100000181, Air Force Office of Scientific Research;
                Award ID: FA9550-19-1-0250
                Funded by: FundRef http://dx.doi.org/10.13039/100000185, Defense Advanced Research Projects Agency;
                Award ID: HR0011-20-2-0046
                Funded by: FundRef http://dx.doi.org/10.13039/501100000781, European Research Council;
                Award ID: ERC-2017-CoG 77164
                Funded by: FundRef http://dx.doi.org/10.13039/501100001711, Swiss National Science Foundation;
                Award ID: Bridge 176563
                Categories
                Research Article
                Physical and Materials Sciences
                SciAdv r-articles
                Optics
                Physics
                Optics
                Custom metadata
                Vivian Hernandez

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