State of the Art and Prospects for Halide Perovskite Nanocrystals

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Abstract

Metal-halide perovskites have rapidly emerged as one of the most promising materials of the 21st century, with many exciting properties and great potential for a broad range of applications, from photovoltaics to optoelectronics and photocatalysis. The ease with which metal-halide perovskites can be synthesized in the form of brightly luminescent colloidal nanocrystals, as well as their tunable and intriguing optical and electronic properties, has attracted researchers from different disciplines of science and technology. In the last few years, there has been a significant progress in the shape-controlled synthesis of perovskite nanocrystals and understanding of their properties and applications. In this comprehensive review, researchers having expertise in different fields (chemistry, physics, and device engineering) of metal-halide perovskite nanocrystals have joined together to provide a state of the art overview and future prospects of metal-halide perovskite nanocrystal research.

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Most cited references 1,337

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Abstract: found
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Organometal halide perovskites as visible-light sensitizers for photovoltaic cells.

Akihiro Kojima, Kenjiro Teshima, Yasuo Shirai … (2009)

Two organolead halide perovskite nanocrystals, CH(3)NH(3)PbBr(3) and CH(3)NH(3)PbI(3), were found to efficiently sensitize TiO(2) for visible-light conversion in photoelectrochemical cells. When self-assembled on mesoporous TiO(2) films, the nanocrystalline perovskites exhibit strong band-gap absorptions as semiconductors. The CH(3)NH(3)PbI(3)-based photocell with spectral sensitivity of up to 800 nm yielded a solar energy conversion efficiency of 3.8%. The CH(3)NH(3)PbBr(3)-based cell showed a high photovoltage of 0.96 V with an external quantum conversion efficiency of 65%.

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Electron-hole diffusion lengths exceeding 1 micrometer in an organometal trihalide perovskite absorber.

Samuel D Stranks, Giles E Eperon, Giulia Grancini … (2013)

Organic-inorganic perovskites have shown promise as high-performance absorbers in solar cells, first as a coating on a mesoporous metal oxide scaffold and more recently as a solid layer in planar heterojunction architectures. Here, we report transient absorption and photoluminescence-quenching measurements to determine the electron-hole diffusion lengths, diffusion constants, and lifetimes in mixed halide (CH3NH3PbI(3-x)Cl(x)) and triiodide (CH3NH3PbI3) perovskite absorbers. We found that the diffusion lengths are greater than 1 micrometer in the mixed halide perovskite, which is an order of magnitude greater than the absorption depth. In contrast, the triiodide absorber has electron-hole diffusion lengths of ~100 nanometers. These results justify the high efficiency of planar heterojunction perovskite solar cells and identify a critical parameter to optimize for future perovskite absorber development.

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Author and article information

Journal

Journal ID (nlm-ta): ACS Nano

Journal ID (iso-abbrev): ACS Nano

Journal ID (publisher-id): nn

Journal ID (coden): ancac3

Title: ACS Nano

Publisher: American Chemical Society

ISSN (Print): 1936-0851

ISSN (Electronic): 1936-086X

Publication date (Electronic): 17 June 2021

Publication date (Print): 27 July 2021

Volume: 15

Issue: 7

Pages: 10775-10981

Affiliations

[1 ]Chair for Photonics and Optoelectronics, Nano-Institute Munich, Department of Physics, Ludwig-Maximilians-Universität (LMU) , Königinstrasse 10, 80539 Munich, Germany

[2 ]Cavendish Laboratory, University of Cambridge , 19 JJ Thomson Avenue, Cambridge CB3 0HE, United Kingdom

[3 ]School of Chemistry, University of Hyderabad , Hyderabad 500 046, India

[4 ]Department of Chemistry, KU Leuven , 3001 Leuven, Belgium

[5 ]Department of Chemical Engineering, Massachusetts Institute of Technology , Cambridge, Massachusetts 02139, United States

[6 ]EMAT, University of Antwerp , Groenenborgerlaan 171, 2020 Antwerp, Belgium

[7 ]NANOlab Center of Excellence, University of Antwerp , 2020 Antwerp, Belgium

[8 ]Department of Chemistry, Indian Institute of Science Education and Research (IISER) , Pune 411008, India

[9 ]School of Science and Technology for Optoelectronic Information ,Yantai University , Yantai, Shandong Province 264005, China

[10 ]Division of Physical Science and Engineering, King Abdullah University of Science and Technology , Thuwal 23955-6900, Kingdom of Saudi Arabia

[11 ]MIIT Key Laboratory of Advanced Display Materials and Devices, Institute of Optoelectronics & Nanomaterials, College of Materials Science and Engineering, Nanjing University of Science and Technology , Nanjing 210094, China

[12 ]Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University , Singapore 637371

[13 ]Department of Chemistry, University of California, Berkeley , Berkeley, California 94720, United States

[14 ]Materials Sciences Division, Lawrence Berkeley National Laboratory , Berkeley, California 94720, United States

[15 ]LUMINOUS! Center of Excellence for Semiconductor Lighting and Displays, TPI-The Photonics Institute, School of Electrical and Electronic Engineering, Nanyang Technological University , Singapore 639798

[16 ]Department of Materials Science and Engineering, University of California , Berkeley, California 94720, United States

[17 ]Institute of Functional Nano & Soft Materials (FUNSOM), Jiangsu Key Laboratory for Carbon-Based Functional Materials and Devices, Soochow University , Suzhou 215123, China

[18 ]Lehrstuhl für Funktionelle Materialien, Physik Department, Technische Universität München , James-Franck-Str. 1, 85748 Garching, Germany

[19 ]Heinz Maier-Leibnitz Zentrum (MLZ), Technische Universität München , Lichtenbergstr. 1, D-85748 Garching, Germany

[20 ]MACS Department of Microbial and Molecular Systems, KU Leuven , 3001 Leuven, Belgium

[21 ]Chemical Physics and NanoLund Lund University , PO Box 124, 22100 Lund, Sweden

[22 ]Graduate School of Environmental Science and Research Institute for Electronic Science, Hokkaido University , Sapporo, Hokkaido 001-0020, Japan

[23 ]Department of Chemistry and Biochemistry, University of California , Santa Cruz, California 95064, United States

[24 ]Beijing Key Laboratory of Nanophotonics and Ultrafine Optoelectronic Systems, School of Materials Science & Engineering, Beijing Institute of Technology , 5 Zhongguancun South Street, Haidian District, Beijing 100081, China

[25 ]Department of Materials Science and Engineering, and Centre for Functional Photonics (CFP), City University of Hong Kong , 83 Tat Chee Avenue, Kowloon, Hong Kong S.A.R.

[26 ]McKetta Department of Chemical Engineering and Texas Materials Institute, The University of Texas at Austin , Austin, Texas 78712-1062, United States

[27 ]School of Materials Sciences, Indian Association for the Cultivation of Science , Kolkata 700032, India

[28 ]Department of Chemistry and Biochemistry, San Diego State University , San Diego, California 92182, United States

[29 ]Department of Chemistry, University of Washington , Seattle, Washington 98195, United States

[30 ]Department of Chemistry, Texas A&M University , College Station, Texas 77843, United States

[31 ]Centre for Disruptive Photonic Technologies (CDPT), Nanyang Technological University , Singapore 637371

[32 ]Division of Physics and Applied Physics, School of Physical and Mathematical Sciences, Nanyang Technological University , Singapore 639798

[33 ]Department of Electrical and Electronics Engineering, Department of Physics, UNAM-Institute of Materials Science and Nanotechnology, Bilkent University , Ankara 06800, Turkey

[34 ]Institute of Advanced Materials (INAM), Universitat Jaume I , 12071 Castelló, Spain

[35 ]Max Planck Institute for Polymer Research , Mainz 55128, Germany

[36 ]National Renewable Energy Laboratory , Golden, Colorado 80401, United States

[37 ]Institute of Molecular Science, University of Valencia , c/Catedrático José Beltrán 2, Paterna, Valencia 46980, Spain

[38 ]School of Environmental Science and Engineering, Shanghai Jiao Tong University , Shanghai 200240, China

[39 ]Nanochemistry Department, Istituto Italiano di Tecnologia , Via Morego 30, Genova 16163, Italy

[40 ]Institute of Inorganic Chemistry and § Institute of Chemical and Bioengineering, Department of Chemistry and Applied Bioscience, ETH Zurich , Vladimir Prelog Weg 1, CH-8093 Zürich, Switzerland

[41 ]Laboratory for Thin Films and Photovoltaics, Empa−Swiss Federal Laboratories for Materials Science and Technology , Überlandstrasse 129, CH-8600 Dübendorf, Switzerland

[42 ]Kavli Energy NanoScience Institute , Berkeley, California 94720, United States

[43 ]Institute for Chemical and Bioengineering, Department of Chemistry and Applied Biosciences, ETH-Zurich , CH-8093 Zürich, Switzerland

[44 ]Notre Dame Radiation Laboratory, Department of Chemistry and Biochemistry, University of Notre Dame , Notre Dame, Indiana 46556, United States

[45 ]Department of Materials Science and Engineering and ARC Centre of Excellence in Future Low-Energy Electronics Technologies (FLEET), Monash University , Clayton, Victoria 3800, Australia

[46 ]Istituto Italiano di Tecnologia , Via Morego 30, 16163 Genova, Italy

[47 ]Department of Chemical Engineering and Biotechnology, University of Cambridge , Cambridge CB3 0AS, United Kingdom

[48 ]Department of Materials, Imperial College London , Exhibition Road, London SW7 2AZ, United Kingdom

[49 ]CINBIO, Universidade de Vigo , Materials Chemistry and Physics group, Departamento de Química Física, Campus Universitario As Lagoas, Marcosende, 36310 Vigo, Spain

[50 ]Advanced Membranes and Porous Materials Center, King Abdullah University of Science and Technology , Thuwal 23955-6900, Kingdom of Saudi Arabia

[51 ]KAUST Catalysis Center, King Abdullah University of Science and Technology , Thuwal 23955-6900, Kingdom of Saudi Arabia

[52 ]Multiscale Crystal Materials Research Center, Shenzhen Institute of Advanced Technology, Chinese Academy of Sciences , Shenzhen 518055, China

Author notes

[* ]Email: r.hoye@ 123456imperial.ac.uk .

[* ]Email: lakshmi@ 123456uvigo.es or l.polavarapu@ 123456lmu.de .

Author information

Amrita Dey https://orcid.org/0000-0003-2372-2172

Apurba De https://orcid.org/0000-0002-3042-0642

Elke Debroye https://orcid.org/0000-0003-1087-4759

Seung Kyun Ha https://orcid.org/0000-0003-2967-1097

Jun Yin https://orcid.org/0000-0002-1749-1120

Mengyu Gao https://orcid.org/0000-0003-1385-7364

Javad Shamsi https://orcid.org/0000-0003-4684-5407

Tushar Debnath https://orcid.org/0000-0002-8108-4482

Muhan Cao https://orcid.org/0000-0002-7988-7219

Manuel A. Scheel https://orcid.org/0000-0003-0508-6694

Sudhir Kumar https://orcid.org/0000-0002-2994-7084

Julian A. Steele https://orcid.org/0000-0001-7982-4413

Yangning Zhang https://orcid.org/0000-0001-5511-955X

Anirban Dutta https://orcid.org/0000-0001-9915-6985

Andrey L. Rogach https://orcid.org/0000-0002-8263-8141

Angshuman Nag https://orcid.org/0000-0003-2308-334X

Anunay Samanta https://orcid.org/0000-0003-1551-0209

Brian A. Korgel https://orcid.org/0000-0001-6242-7526

Chih-Jen Shih https://orcid.org/0000-0002-5258-3485

Daniel R. Gamelin https://orcid.org/0000-0003-2888-9916

Haibo Zeng https://orcid.org/0000-0002-0281-3617

Haizheng Zhong https://orcid.org/0000-0002-2662-7472

Handong Sun https://orcid.org/0000-0002-2261-7103

Hilmi Volkan Demir https://orcid.org/0000-0003-1793-112X

Ivan G. Scheblykin https://orcid.org/0000-0001-6059-4777

Iván Mora-Seró https://orcid.org/0000-0003-2508-0994

Jacek K. Stolarczyk https://orcid.org/0000-0001-7935-4204

Jin Z. Zhang https://orcid.org/0000-0003-3437-912X

Johan Hofkens https://orcid.org/0000-0002-9101-0567

Joseph M. Luther https://orcid.org/0000-0002-4054-8244

Julia Pérez-Prieto https://orcid.org/0000-0002-5833-341X

Liang Li https://orcid.org/0000-0003-3898-0641

Liberato Manna https://orcid.org/0000-0003-4386-7985

Maryna I. Bodnarchuk https://orcid.org/0000-0001-6597-3266

Maksym V. Kovalenko https://orcid.org/0000-0002-6396-8938

Maarten B. J. Roeffaers https://orcid.org/0000-0001-6582-6514

Narayan Pradhan https://orcid.org/0000-0003-4646-8488

Omar F. Mohammed https://orcid.org/0000-0001-8500-1130

Osman M. Bakr https://orcid.org/0000-0002-3428-1002

Peidong Yang https://orcid.org/0000-0003-4799-1684

Peter Müller-Buschbaum https://orcid.org/0000-0002-9566-6088

Prashant V. Kamat https://orcid.org/0000-0002-2465-6819

Qiaoliang Bao https://orcid.org/0000-0002-6971-789X

Qiao Zhang https://orcid.org/0000-0001-9682-3295

Roman Krahne https://orcid.org/0000-0003-0066-7019

Raquel E. Galian https://orcid.org/0000-0001-8703-4403

Samuel D. Stranks https://orcid.org/0000-0002-8303-7292

Sara Bals https://orcid.org/0000-0002-4249-8017

Vasudevanpillai Biju https://orcid.org/0000-0003-3650-9637

William A. Tisdale https://orcid.org/0000-0002-6615-5342

Robert L. Z. Hoye https://orcid.org/0000-0002-7675-0065

Lakshminarayana Polavarapu https://orcid.org/0000-0002-9040-5719

Article

DOI: 10.1021/acsnano.0c08903

PMC ID: 8482768

PubMed ID: 34137264

SO-VID: 5fb93be3-562e-4b93-a6b3-6689c4be1b2b

License:

Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained ( https://creativecommons.org/licenses/by/4.0/).

History

Date received : 16 December 2020

Date accepted : 04 May 2021

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document-id-old-9 nn0c08903

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ScienceOpen disciplines: Nanotechnology

Keywords: metal-halide perovskite nanocrystals,perovskite nanoplatelets,perovskite nanocubes,perovskite nanowires,lead-free perovskite nanocrystals,light-emitting devices,photovoltaics,lasers,photocatalysts,photodetectors

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ScienceOpen disciplines: Nanotechnology

Keywords: metal-halide perovskite nanocrystals, perovskite nanoplatelets, perovskite nanocubes, perovskite nanowires, lead-free perovskite nanocrystals, light-emitting devices, photovoltaics, lasers, photocatalysts, photodetectors

State of the Art and Prospects for Halide Perovskite Nanocrystals

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Most cited references 1,337

Organometal halide perovskites as visible-light sensitizers for photovoltaic cells.

Issues and challenges facing rechargeable lithium batteries.

Electron-hole diffusion lengths exceeding 1 micrometer in an organometal trihalide perovskite absorber.

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