Spin Liquid Ground State of the $S=1/2$ Kagome Heisenberg Model

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Abstract

Condensed matter physicists have long sought a realistic two-dimensional (2D) magnetic system whose ground state is a {\it spin liquid}---a zero temperature state in which quantum fluctuations have melted away any form of magnetic order. The nearest-neighbor $S=1/2$ Heisenberg model on the kagome lattice has seemed an ideal candidate, but in recent years some approximate numerical approaches to it have yielded instead a valence bond crystal. We have used the density matrix renormalization group to perform very accurate simulations on numerous cylinders with circumferences up to 12 lattice spacings, finding instead of the valence bond crystal a singlet-gapped spin liquid with substantially lower energy that appears to have $Z_2$ topological order. Our results, through a combination of very low energy, short correlation lengths and corresponding small finite size effects, a new rigorous energy bound, and consistent behavior on many cylinders, provide strong evidence that the 2D ground state of this model is a gapped spin liquid.

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Quantum spin-liquid emerging in two-dimensional correlated Dirac fermions

A Muramatsu, F. Assaad, T. Lang … (2010)

At sufficiently low temperatures, condensed-matter systems tend to develop order. An exception are quantum spin-liquids, where fluctuations prevent a transition to an ordered state down to the lowest temperatures. While such states are possibly realized in two-dimensional organic compounds, they have remained elusive in experimentally relevant microscopic two-dimensional models. Here, we show by means of large-scale quantum Monte Carlo simulations of correlated fermions on the honeycomb lattice, a structure realized in graphene, that a quantum spin-liquid emerges between the state described by massless Dirac fermions and an antiferromagnetically ordered Mott insulator. This unexpected quantum-disordered state is found to be a short-range resonating valence bond liquid, akin to the one proposed for high temperature superconductors. Therefore, the possibility of unconventional superconductivity through doping arises. We foresee its realization with ultra-cold atoms or with honeycomb lattices made with group IV elements.