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      3D Janus plasmonic helical nanoapertures for polarization-encrypted data storage

      research-article
      , ,
      Light, Science & Applications
      Nature Publishing Group UK
      Metamaterials, Photonic devices

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          Abstract

          Helical structures have attracted considerable attention due to their inherent optical chirality. Here, we report a unique type of 3D Janus plasmonic helical nanoaperture with direction-controlled polarization sensitivity, which is simply fabricated via the one-step grayscale focused ion beam milling method. Circular dichroism in transmission of as large as 0.72 is experimentally realized in the forward direction due to the spin-dependent mode coupling process inside the helical nanoaperture. However, in the backward direction, the nanoaperture acquires giant linear dichroism in transmission of up to 0.87. By encoding the Janus metasurface with the two nanoaperture enantiomers having specified rotation angles, direction-controlled polarization-encrypted data storage is demonstrated for the first time, where a binary quick-response code image is displayed in the forward direction under the circularly polarized incidence of a specified handedness, while a distinct grayscale image is revealed in the backward direction under linearly polarized illumination with a specified azimuthal angle. We envision that the proposed Janus helical nanoapertures will provide an appealing platform for a variety of applications, which will range from multifunctional polarization control, enantiomer sensing, data encryption and decryption to optical information processing.

          Data storage: Helical holes for polarized encryption

          Tiny helical apertures etched in gold could act as unit cells for data storage technologies based on the manipulation of polarized light. Helical nanostructures are suited to storing binary data because they exist in two forms, left- and right-handed helixes. Xiaodong Yang, Jie Gao and Yang Chen at Missouri University of Science and Technology used ion beam milling to carve arrays of helter-skelter-shaped helical ‘nanoapertures’ in 180-nanometer-thick gold films. Their samples allow selective transmission of certain types of polarized light, while blocking others. Moreover, this polarization sensitivity depends on the direction of the incoming light, meaning that when light is directed in one direction the array produces binary images such as QR codes, while in the other direction it can reproduce grayscale photographs. This opens exciting possibilities for data encryption and optical information processing.

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          Most cited references35

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          Protein folding and misfolding.

          The manner in which a newly synthesized chain of amino acids transforms itself into a perfectly folded protein depends both on the intrinsic properties of the amino-acid sequence and on multiple contributing influences from the crowded cellular milieu. Folding and unfolding are crucial ways of regulating biological activity and targeting proteins to different cellular locations. Aggregation of misfolded proteins that escape the cellular quality-control mechanisms is a common feature of a wide range of highly debilitating and increasingly prevalent diseases.
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            Gold helix photonic metamaterial as broadband circular polarizer.

            We investigated propagation of light through a uniaxial photonic metamaterial composed of three-dimensional gold helices arranged on a two-dimensional square lattice. These nanostructures are fabricated via an approach based on direct laser writing into a positive-tone photoresist followed by electrochemical deposition of gold. For propagation of light along the helix axis, the structure blocks the circular polarization with the same handedness as the helices, whereas it transmits the other, for a frequency range exceeding one octave. The structure is scalable to other frequency ranges and can be used as a compact broadband circular polarizer.
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              Twisted optical metamaterials for planarized ultrathin broadband circular polarizers.

              Optical metamaterials are usually based on planarized, complex-shaped, resonant nano-inclusions. Three-dimensional geometries may provide a wider set of functionalities, including broadband chirality to manipulate circular polarization at the nanoscale, but their fabrication becomes challenging as their dimensions get smaller. Here we introduce a new paradigm for the realization of optical metamaterials, showing that three-dimensional effects may be obtained without complicated inclusions, but instead by tailoring the relative orientation within the lattice. We apply this concept to realize planarized, broadband bianisotropic metamaterials as stacked nanorod arrays with a tailored rotational twist. Because of the coupling among closely spaced twisted plasmonic metasurfaces, metamaterials realized with conventional lithography may effectively operate as three-dimensional helical structures with broadband bianisotropic optical response. The proposed concept is also shown to relax alignment requirements common in three-dimensional metamaterial designs. The realized sample constitutes an ultrathin, broadband circular polarizer that may be directly integrated within nanophotonic systems.
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                Author and article information

                Contributors
                +1 (573) 341-6273 , yangxia@mst.edu
                +1 (573) 341-6516 , gaojie@mst.edu
                Journal
                Light Sci Appl
                Light Sci Appl
                Light, Science & Applications
                Nature Publishing Group UK (London )
                2095-5545
                2047-7538
                15 May 2019
                15 May 2019
                2019
                : 8
                : 45
                Affiliations
                ISNI 0000 0000 9364 6281, GRID grid.260128.f, Department of Mechanical and Aerospace Engineering, , Missouri University of Science and Technology, ; Rolla, MO 65409 USA
                Author information
                http://orcid.org/0000-0001-9031-3155
                Article
                156
                10.1038/s41377-019-0156-8
                6517422
                31098013
                76b28221-6538-4c52-8fc0-79725a5d49fa
                © The Author(s) 2019

                Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.

                History
                : 11 February 2019
                : 16 April 2019
                : 24 April 2019
                Funding
                Funded by: FundRef https://doi.org/10.13039/100007297, United States Department of Defense | United States Navy | ONR | Office of Naval Research Global (ONR Global);
                Award ID: N00014-16-1-2408
                Award Recipient :
                Funded by: FundRef https://doi.org/10.13039/100000001, National Science Foundation (NSF);
                Award ID: DMR-1552871
                Award ID: ECCS-1653032
                Award Recipient :
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                © The Author(s) 2019

                metamaterials,photonic devices
                metamaterials, photonic devices

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