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      Configuration and Performance of a Mobile 129Xe Polarizer

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      , ,
      Applied Magnetic Resonance
      Springer Vienna

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          Abstract

          A stand-alone, self-contained and transportable system for the polarization of 129Xe by spin exchange optical pumping with Rb is described. This mobile polarizer may be operated in batch or continuous flow modes with medium amounts of hyperpolarized 129Xe for spectroscopic or small animal applications. A key element is an online nuclear magnetic resonance module which facilitates continuous monitoring of polarization generation in the pumping cell as well as the calculation of the absolute 129Xe polarization. The performance of the polarizer with respect to the crucial parameters temperature, xenon and nitrogen partial pressures, and the total gas flow is discussed. In batch mode the highest 129Xe polarization of P Xe = 40 % was achieved using 0.1 mbar xenon partial pressure. For a xenon flow of 6.5 and 26 mln/min, P Xe = 25 % and P Xe = 13 % were reached, respectively. The mobile polarizer may be a practical and efficient means to make the applicability of hyperpolarized 129Xe more widespread.

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          Most cited references35

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          Spin-exchange optical pumping of noble-gas nuclei

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            Nuclear magnetic resonance of laser-polarized noble gases in molecules, materials, and organisms.

            The sensitivity of conventional nuclear magnetic resonance (NMR) techniques is fundamentally limited by the ordinarily low spin polarization achievable in even the strongest NMR magnets. However, by transferring angular momentum from laser light to electronic and nuclear spins, optical pumping methods can increase the nuclear spin polarization of noble gases by several orders of magnitude, thereby greatly enhancing their NMR sensitivity. This review describes the principles and magnetic resonance applications of laser-polarized noble gases. The enormous sensitivity enhancement afforded by optical pumping can be exploited to permit a variety of novel NMR experiments across numerous disciplines. Many such experiments are reviewed, including the void-space imaging of organisms and materials, NMR and MRI of living tissues, probing structure and dynamics of molecules in solution and on surfaces, NMR sensitivity enhancement via polarization transfer, and low-field NMR and MRI. (c) 2002 Elsevier Science (USA).
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              Is Open Access

              Controlling the Spontaneous Emission Rate of Monolayer MoS\(_2\) in a Photonic Crystal Nanocavity

              We report on controlling the spontaneous emission (SE) rate of a molybdenum disulfide (MoS\(_2\)) monolayer coupled with a planar photonic crystal (PPC) nanocavity. Spatially resolved photoluminescence (PL) mapping shows strong variations of emission when the MoS\(_2\) monolayer is on the PPC cavity, on the PPC lattice, on the air gap, and on the unpatterned gallium phosphide substrate. Polarization dependences of the cavity-coupled MoS\(_2\) emission show a more than 5 times stronger extracted PL intensity than the un-coupled emission, which indicates an underlying cavity mode Purcell enhancement of MoS\(_2\) SE rate exceeding a factor of 70.
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                Author and article information

                Contributors
                +49-30-34817952 , +49-30-34817507 , wolfgang.kilian@ptb.de
                Journal
                Appl Magn Reson
                Appl Magn Reson
                Applied Magnetic Resonance
                Springer Vienna (Vienna )
                0937-9347
                1613-7507
                10 November 2012
                10 November 2012
                February 2013
                : 44
                : 1-2
                : 65-80
                Affiliations
                Physikalisch-Technische Bundesanstalt, Abbestr. 2-12, 10587 Berlin, Germany
                Article
                425
                10.1007/s00723-012-0425-7
                3549238
                23349565
                aa8ed53f-e021-4618-9e4e-cc081686465a
                © The Author(s) 2012
                History
                : 17 August 2012
                : 17 October 2012
                Categories
                Article
                Custom metadata
                © Springer-Verlag Wien 2013

                Radiology & Imaging
                Radiology & Imaging

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