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      • Record: found
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      Recent developments in gold-catalyzed cycloaddition reactions

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      Author(s): 1 , , 2 ,
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      Publication date (Electronic):
      Journal: Beilstein Journal of Organic Chemistry
      Publisher: Beilstein-Institut
      Keywords: alkene, alkyne, allene, catalysis, cycloaddition, gold

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          Summary

          In the last years there have been extraordinary advances in the development of gold-catalyzed cycloaddition processes. In this review we will summarize some of the most remarkable examples, and present the mechanistic rational underlying the transformations.

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          Ligand effects in homogeneous Au catalysis.

          David J Gorin, Benjamin D Sherry, F Dean Toste (2008)
          Article 0 comments Cited 477 times – based on 0 reviews     Review now
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            Relativistic effects in homogeneous gold catalysis.

            David J Gorin, F Dean Toste (2007)
            Transition-metal catalysts containing gold present new opportunities for chemical synthesis, and it is therefore not surprising that these complexes are beginning to capture the attention of the chemical community. Cationic phosphine-gold(i) complexes are especially versatile and selective catalysts for a growing number of synthetic transformations. The reactivity of these species can be understood in the context of theoretical studies on gold; relativistic effects are especially helpful in rationalizing the reaction manifolds available to gold catalysts. This Review draws on experimental and computational data to present our current understanding of homogeneous gold catalysis, focusing on previously unexplored reactivity and its application to the development of new methodology.
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              Gold and platinum catalysis--a convenient tool for generating molecular complexity.

              Alois Fürstner (2009)
              This critical review intends to familiarize the reader with the essence of pi-acid catalysis, in particular with reactions or reaction cascades effected by gold and platinum complexes. Even though materialized in apparently different reactivity modes, such noble metal catalyzed processes can be easily rationalized on the basis of a uniform mechanistic scheme that is outlined in detail. The resulting increase in molecular complexity is illustrated by selected natural product total syntheses and the formation of various intricate non-natural compounds (106 references).
              Article 0 comments Cited 261 times – based on 0 reviews     Review now
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                Author and article information

                Contributors
                Fernando López
                José L Mascareñas
                F Dean Toste: Role: Guest Editor
                Journal
                Journal ID (nlm-ta): Beilstein J Org Chem
                Title: Beilstein Journal of Organic Chemistry
                Publisher: Beilstein-Institut (Trakehner Str. 7-9, 60487 Frankfurt am Main, Germany )
                ISSN (Electronic): 1860-5397
                Publication date Collection: 2011
                Publication date (Electronic): 9 August 2011
                Volume: 7
                Pages: 1075-1094
                Affiliations
                [1 ]Instituto de Química Orgánica General, CSIC, C/ Juan de la Cierva 3, 28006, Madrid, Spain, (+) 34 915622900, Fax: (+) 34 915644853
                [2 ]Departamento de Química Orgánica, Centro Singular de Investigación en Química Biológica y Materiales Moleculares, y Unidad Asociada al CSIC. Universidad de Santiago de Compostela, Avda. de las Ciencias, s/n, 15782, Santiago de Compostela, Spain, (+) 34 981563100 Fax: (+) 34 981595012
                Article
                DOI: 10.3762/bjoc.7.124
                PMC ID: 3167873
                PubMed ID: 21915211
                SO-VID: e5fe57f7-8332-400b-b995-9245009c8a21
                Copyright © Copyright © 2011, López and Mascareñas; licensee Beilstein-Institut.
                License:

                This is an Open Access article under the terms of the Creative Commons Attribution License ( http://creativecommons.org/licenses/by/2.0), which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.

                The license is subject to the Beilstein Journal of Organic Chemistry terms and conditions: ( http://www.beilstein-journals.org/bjoc)

                History
                Date received : 16 May 2011
                Date accepted : 14 July 2011
                Categories
                Subject: Review
                Subject: Chemistry
                Subject: Organic Chemistry

                ScienceOpen disciplines: Organic & Biomolecular chemistry
                Keywords: alkene,alkyne,allene,catalysis,cycloaddition,gold
                Data availability:
                ScienceOpen disciplines: Organic & Biomolecular chemistry
                Keywords: alkene, alkyne, allene, catalysis, cycloaddition, gold

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