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      Single-Frame Characterization of Ultrafast Pulses with Spatiotemporal Orbital Angular Momentum

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          Abstract

          Light that carries spatiotemporal orbital angular momentum (ST-OAM) makes possible new types of optical vortices arising from transverse OAM. ST-OAM pulses exhibit novel properties during propagation, transmission, refraction, diffraction, and nonlinear conversion, attracting growing experimental and theoretical interest and studies. However, one major challenge is the lack of a simple and straightforward method for characterizing ultrafast ST-OAM pulses. Using spatially resolved spectral interferometry, we demonstrate a simple, stationary, single-frame method to quantitatively characterize ultrashort light pulses carrying ST-OAM. Using our method, the presence of an ST-OAM pulse, including its main characteristics such as topological charge numbers and OAM helicity, can be identified easily from the unique and unambiguous features directly seen on the raw data—without any need for a full analysis of the data. After processing and reconstructions, other exquisite features, including pulse dispersion and beam divergence, can also be fully characterized. Our fast characterization method allows high-throughput and quick feedback during the generation and optical alignment processes of ST-OAM pulses. It is straightforward to extend our method to single-shot measurement by using a high-speed camera that matches the pulse repetition rate. This new method can help advance the field of spatially and temporally structured light and its applications in advanced metrologies.

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          Most cited references35

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          Controlled rotation of optically trapped microscopic particles.

          We demonstrate controlled rotation of optically trapped objects in a spiral interference pattern. This pattern is generated by interfering an annular shaped laser beam with a reference beam. Objects are trapped in the spiral arms of the pattern. Changing the optical path length causes this pattern, and thus the trapped objects, to rotate. Structures of silica microspheres, microscopic glass rods, and chromosomes are set into rotation at rates in excess of 5 hertz. This technique does not depend on intrinsic properties of the trapped particle and thus offers important applications in optical and biological micromachines.
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            Optical vortices

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              Transverse and longitudinal angular momenta of light

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                Author and article information

                Journal
                ACS Photonics
                ACS Photonics
                ph
                apchd5
                ACS Photonics
                American Chemical Society
                2330-4022
                23 July 2022
                17 August 2022
                : 9
                : 8
                : 2802-2808
                Affiliations
                []JILA and Department of Physics, University of Colorado and NIST , 440 UCB, Boulder, Colorado 80309, United States
                []KMLabs Inc. , 4775 Walnut Street, Suite 102, Boulder, Colorado 80301, United States
                Author notes
                Author information
                https://orcid.org/0000-0002-3423-277X
                Article
                10.1021/acsphotonics.2c00626
                9389650
                35996367
                f7fcf40c-a5bf-4eab-8ba0-787a576731af
                © 2022 The Authors. Published by American Chemical Society

                Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works ( https://creativecommons.org/licenses/by-nc-nd/4.0/).

                History
                : 26 April 2022
                Funding
                Funded by: Division of Graduate Education, doi 10.13039/100000082;
                Award ID: DGE-1650115
                Funded by: Basic Energy Sciences, doi 10.13039/100006151;
                Award ID: DE-FG02-99ER14982
                Funded by: Air Force Office of Scientific Research, doi 10.13039/100000181;
                Award ID: FA9550-16-1-0121
                Categories
                Article
                Custom metadata
                ph2c00626
                ph2c00626

                orbital angular momentum,spatiotemporal optical vortex,single shot,spectral interferometer,imaging spectrometer,ultrafast vortex pulses,spatiotemporally sculptured light fields,space-time wave packets

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