Nonlinear Exciton‐Mie Coupling in Transition Metal Dichalcogenide Nanoresonators

Subwavelength optical resonators made of high-index dielectric materials provide efficient ways to manipulate light at the nanoscale through mode interferences and enhancement of both electric and magnetic fields. Such Mie-resonant dielectric structures have low absorption, and their functionalities are limited predominantly by radiative losses. We implement a new physical mechanism for suppressing radiative losses of individual nanoscale resonators to engineer special modes with high quality factors: optical bound states in the continuum (BICs). We demonstrate that an individual subwavelength dielectric resonator hosting a BIC mode can boost nonlinear effects increasing second-harmonic generation efficiency. Our work suggests a route to use subwavelength high-index dielectric resonators for a strong enhancement of light–matter interactions with applications to nonlinear optics, nanoscale lasers, quantum photonics, and sensors.

Observations of high-harmonic generation from a single layer of a transition metal dichalcogenide opens the door to studying strong-field and attosecond phenomena in two-dimensional materials.