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      Potassium isotope anomalies in meteorites inherited from the protosolar molecular cloud

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      Science Advances
      American Association for the Advancement of Science

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          Abstract

          Potassium, a moderately volatile element, shows presolar isotopic heterogeneity in meteorites.

          Abstract

          Potassium (K) and other moderately volatile elements are depleted in many solar system bodies relative to CI chondrites, which closely match the composition of the Sun. These depletions and associated isotopic fractionations were initially believed to result from thermal processing in the protoplanetary disk, but so far, no correlation between the K depletion and its isotopic composition has been found. Our new high-precision K isotope data correlate with other neutron-rich nuclides (e.g., 64Ni and 54Cr) and suggest that the observed 41K variations have a nucleosynthetic origin. We propose that K isotope anomalies are inherited from an isotopically heterogeneous protosolar molecular cloud, and were preserved in bulk primitive meteorites. Thus, the heterogeneous distribution of both refractory and moderately volatile elements in chondritic meteorites points to a limited radial mixing in the protoplanetary disk.

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          Most cited references133

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          Solar System Abundances and Condensation Temperatures of the Elements

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            Abundances of the elements: Meteoritic and solar

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              142Nd evidence for early (>4.53 Ga) global differentiation of the silicate Earth.

              New high-precision samarium-neodymium isotopic data for chondritic meteorites show that their 142Nd/144Nd ratio is 20 parts per million lower than that of most terrestrial rocks. This difference indicates that most (70 to 95%) of Earth's mantle is compositionally similar to the incompatible element-depleted source of mid-ocean ridge basalts, possibly as a result of a global differentiation 4.53 billion years ago (Ga), within 30 million years of Earth's formation. The complementary enriched reservoir has never been sampled and is probably located at the base of the mantle. These data influence models of Earth's compositional structure and require revision of the timing of global differentiation on Earth's Moon and Mars.
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                Author and article information

                Journal
                Sci Adv
                Sci Adv
                SciAdv
                advances
                Science Advances
                American Association for the Advancement of Science
                2375-2548
                October 2020
                09 October 2020
                : 6
                : 41
                : eabd0511
                Affiliations
                Department of Earth and Planetary Sciences, Harvard University, 20 Oxford Street, Cambridge, MA 02138, USA.
                Author notes
                [* ]Corresponding author. Email: yku@ 123456g.harvard.edu
                Author information
                http://orcid.org/0000-0003-1869-7339
                Article
                abd0511
                10.1126/sciadv.abd0511
                7546711
                33036981
                6498e4a0-ed73-4ee6-9b4d-3e4c0417900b
                Copyright © 2020 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC).

                This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license, which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited.

                History
                : 28 May 2020
                : 19 August 2020
                Funding
                Funded by: NASA Emerging Worlds Program grant;
                Award ID: 80NSSC20K0346
                Categories
                Research Article
                Research Articles
                SciAdv r-articles
                Planetary Science
                Custom metadata
                Kyle Solis

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