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      Polyoxometalate Modified Separator for Performance Enhancement of Magnesium–Sulfur Batteries

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          Most cited references62

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          Quest for nonaqueous multivalent secondary batteries: magnesium and beyond.

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            Metal–organic framework-based separator for lithium–sulfur batteries

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              Lithium sulfur batteries, a mechanistic review

              Lithium sulfur batteries, review of current mechanistic understanding and the gap between experimentally derived mechanisms and those used for modelling. Lithium sulfur (Li–S) batteries are one of the most promising next generation battery chemistries with potential to achieve 500–600 W h kg −1 in the next few years. Yet understanding the underlying mechanisms of operation remains a major obstacle to their continued improvement. From a review of a range of analytical studies and physical models, it is clear that experimental understanding is well ahead of state-of-the-art models. Yet this understanding is still hindered by the limitations of available techniques and the implications of experiment and cell design on the mechanism. The mechanisms at the core of physical models for Li–S cells are overly simplistic compared to the latest thinking based upon experimental results, but creating more complicated models will be difficult, due to the lack of and inability to easily measure the necessary parameters. Despite this, there are significant opportunities to improve models with the latest experimentally derived mechanisms. Such models can inform materials research and lead to improved high fidelity models for controls and application engineers.
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                Author and article information

                Contributors
                (View ORCID Profile)
                Journal
                Advanced Functional Materials
                Adv. Funct. Mater.
                Wiley
                1616-301X
                1616-3028
                June 2021
                March 29 2021
                June 2021
                : 31
                : 26
                : 2100868
                Affiliations
                [1 ]Helmholtz Institute Ulm (HIU) Electrochemical Energy Storage Helmholtzstrasse 11 Ulm D‐89081 Germany
                [2 ]Institute for Applied Materials‐Energy Storage Systems (IAM‐ESS) Karlsruhe Institute of Technology (KIT) Hermann‐von‐Helmholtz‐Platz 1 Eggenstein‐Leopoldshafen D‐76344 Germany
                [3 ]Karlsruhe Nano Micro Facility (KNMF) Karlsruhe Institute of Technology (KIT) Hermann‐von‐Helmholtz‐Platz 1 Eggenstein‐Leopoldshafen D‐76344 Germany
                [4 ]Institute of Nanotechnology (INT) Karlsruhe Institute of Technology (KIT) Hermann‐von‐Helmholtz Platz 1 Eggenstein‐Leopoldshafen D‐76344 Germany
                Article
                10.1002/adfm.202100868
                79f12c2a-bd22-41f3-af9c-c28e30598954
                © 2021

                http://creativecommons.org/licenses/by/4.0/

                http://doi.wiley.com/10.1002/tdm_license_1.1

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