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      Na 4Mn 9O 18/Carbon Nanotube Composite as a High Electrochemical Performance Material for Aqueous Sodium-Ion Batteries

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          Abstract

          The aqueous sodium-ion battery (ASIB) is one of the promising new energy storage systems owing to the abundant resources of sodium as well as efficiency and safety of electrolyte. Herein, we report an ASIB system with Na 4Mn 9O 18/carbon nanotube (NMO/CNT) as cathode, metal Zn as anode and a novel Na +/Zn 2+ mixed ion as electrolyte. The NMO/CNT with microspherical structure is prepared by a simple spray-drying method. The prepared battery delivers a high reversible specific capacity and stable cyclability. Furthermore, the battery displays a stable reversible discharge capacity of 53.2 mAh g −1 even at a high current rate of 4 C after 150 cycles. Our results confirm that the NMO/CNT composite is a promising electrode cathode material for ASIBs.

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          Rechargeable lithium batteries with aqueous electrolytes.

          W. Li, J. Dahn, D Wainwright (1994)
          Rechargeable lithium-ion batteries that use an aqueous electrolyte have been developed. Cells with LiMn(2)O(4) and VO(2)(B) as electrodes and 5 M LiNO(3) in water as the electrolyte provide a fundamentally safe and cost-effective technology that can compete with nickelcadmium and lead-acid batteries on the basis of stored energy per unit of weight.
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            Raising the cycling stability of aqueous lithium-ion batteries by eliminating oxygen in the electrolyte.

            Jia-Yan Luo, Wang-Jun Cui, Ping He … (2010)
            Aqueous lithium-ion batteries may solve the safety problem associated with lithium-ion batteries that use highly toxic and flammable organic solvents, and the poor cycling life associated with commercialized aqueous rechargeable batteries such as lead-acid and nickel-metal hydride systems. But all reported aqueous lithium-ion battery systems have shown poor stability: the capacity retention is typically less than 50% after 100 cycles. Here, the stability of electrode materials in an aqueous electrolyte was extensively analysed. The negative electrodes of aqueous lithium-ion batteries in a discharged state can react with water and oxygen, resulting in capacity fading upon cycling. By eliminating oxygen, adjusting the pH values of the electrolyte and using carbon-coated electrode materials, LiTi(2)(PO(4))(3)/Li(2)SO(4)/LiFePO(4) aqueous lithium-ion batteries exhibited excellent stability with capacity retention over 90% after 1,000 cycles when being fully charged/discharged in 10 minutes and 85% after 50 cycles even at a very low current rate of 8 hours for a full charge/discharge offering an energy storage system with high safety, low cost, long cycling life and appropriate energy density.
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              Reversible sodium ion insertion in single crystalline manganese oxide nanowires with long cycle life.

              Yuliang Cao, Lifen Xiao, Wei Wang … (2011)
              Article 0 comments Cited 223 times – based on 0 reviews     Review now
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                Author and article information

                Contributors
                Fuxing Yin: fordjp@163.com
                Zhengjun Liu: lzj125@126.com
                Shuang Yang: 15522560785@163.com
                Zhenzhen Shan: 390881076@qq.com
                Yan Zhao: yanzhao1984@hebut.edu.cn
                Yuting Feng: 372392352@qq.com
                Chengwei Zhang: zhangpan0411@sina.com
                Zhumabay Bakenov: zbakenov@nu.edu.kz
                Journal
                Journal ID (nlm-ta): Nanoscale Res Lett
                Journal ID (iso-abbrev): Nanoscale Res Lett
                Title: Nanoscale Research Letters
                Publisher: Springer US (New York )
                ISSN (Print): 1931-7573
                ISSN (Electronic): 1556-276X
                Publication date (Electronic): 17 October 2017
                Publication date PMC-release: 17 October 2017
                Publication date Collection: 2017
                Volume: 12
                Electronic Location Identifier: 569
                Affiliations
                [1 ]ISNI 0000 0000 9226 1013, GRID grid.412030.4, School of Materials Science & Engineering, Research Institute for Energy Equipment Materials, Tianjin Key Laboratory of Materials Laminating Fabrication and Interface Control Technology, , Hebei University of Technology, ; Tianjin, 300130 China
                [2 ]Synergy Innovation Institute of GDUT, Heyuan, Guangdong Province China
                [3 ]GRID grid.428191.7, School of Engineering, , Nazarbayev University, ; Kabanbay Batyr Ave. 53, Astana, Kazakhstan 010000
                Article
                Publisher ID: 2340
                DOI: 10.1186/s11671-017-2340-1
                PMC ID: 5645269
                PubMed ID: 29043527
                SO-VID: 8e377af7-b017-4eee-ba8a-6e637a52671c
                Copyright © © The Author(s). 2017
                License:

                Open AccessThis article is distributed under the terms of the Creative Commons Attribution 4.0 International License ( http://creativecommons.org/licenses/by/4.0/), which permits unrestricted use, distribution, and reproduction in any medium, provided you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made.

                History
                Date received : 10 August 2017
                Date accepted : 9 October 2017
                Funding
                Funded by: FundRef http://dx.doi.org/10.13039/501100001809, National Natural Science Foundation of China;
                Award ID: 21406052
                Award ID: 21606068
                Award Recipient :
                Funded by: FundRef http://dx.doi.org/10.13039/501100005952, Ministry of Human Resources and Social Security;
                Award ID: CG2015003002
                Funded by: Program for the Outstanding Young Talents of Hebei Province
                Award ID: BJ2014010
                Funded by: Scientific Innovation Grant for Excellent Young Scientists of Hebei University of Technology
                Award ID: 2015001
                Award Recipient :
                Categories
                Subject: Nano Express
                Custom metadata
                issue-copyright-statement © The Author(s) 2017

                ScienceOpen disciplines: Nanomaterials
                Keywords: aqueous sodium-ion battery,cathode,na4mn9o18/carbon nanotube,energy storage and conversion
                Data availability:
                ScienceOpen disciplines: Nanomaterials
                Keywords: aqueous sodium-ion battery, cathode, na4mn9o18/carbon nanotube, energy storage and conversion

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