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      Spatial and frequency-selective optical field coupling absorption in an ultra-thin random metasurface

      , , , ,
      Optics Letters
      Optica Publishing Group

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          Abstract

          Simplified thin-film structures with the capability of spatial and frequency-selective optical field coupling and absorption are desirable for nanophotonics. Herein, we demonstrate the configuration of a 200-nm-thick random metasurface formed by refractory metal nanoresonators, showing near-unity absorption (absorptivity > 90%) covering the visible and near-infrared range (0.380–1.167 µm). Importantly, the resonant optical field is observed to be concentrated in different spatial areas according to different frequencies, paving a feasible way to artificially manipulate spatial coupling and optical absorption via the spectral frequency. The methods and conclusions derived in this work are applicable throughout a wide energy range and hold applications for frequency-selective nanoscale optical field manipulation.

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          Perfect metamaterial absorber.

          We present the design for an absorbing metamaterial (MM) with near unity absorbance A(omega). Our structure consists of two MM resonators that couple separately to electric and magnetic fields so as to absorb all incident radiation within a single unit cell layer. We fabricate, characterize, and analyze a MM absorber with a slightly lower predicted A(omega) of 96%. Unlike conventional absorbers, our MM consists solely of metallic elements. The substrate can therefore be optimized for other parameters of interest. We experimentally demonstrate a peak A(omega) greater than 88% at 11.5 GHz.
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            Solar-driven interfacial evaporation

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              Localized surface plasmon resonance spectroscopy and sensing.

              Localized surface plasmon resonance (LSPR) spectroscopy of metallic nanoparticles is a powerful technique for chemical and biological sensing experiments. Moreover, the LSPR is responsible for the electromagnetic-field enhancement that leads to surface-enhanced Raman scattering (SERS) and other surface-enhanced spectroscopic processes. This review describes recent fundamental spectroscopic studies that reveal key relationships governing the LSPR spectral location and its sensitivity to the local environment, including nanoparticle shape and size. We also describe studies on the distance dependence of the enhanced electromagnetic field and the relationship between the plasmon resonance and the Raman excitation energy. Lastly, we introduce a new form of LSPR spectroscopy, involving the coupling between nanoparticle plasmon resonances and adsorbate molecular resonances. The results from these fundamental studies guide the design of new sensing experiments, illustrated through applications in which researchers use both LSPR wavelength-shift sensing and SERS to detect molecules of chemical and biological relevance.
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                Author and article information

                Contributors
                Journal
                OPLEDP
                Optics Letters
                Opt. Lett.
                Optica Publishing Group
                0146-9592
                1539-4794
                2023
                2023
                March 20 2023
                April 01 2023
                : 48
                : 7
                : 1586
                Article
                10.1364/OL.486017
                d4bc1437-50ed-4a2b-adbc-4228d31e68b6
                © 2023

                https://doi.org/10.1364/OA_License_v2#VOR

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