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      Purcell Enhancement of Erbium Ions in TiO 2 on Silicon Nanocavities

      rapid-communication

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          Abstract

          Isolated solid-state atomic defects with telecom optical transitions are ideal quantum photon emitters and spin qubits for applications in long-distance quantum communication networks. Prototypical telecom defects, such as erbium, suffer from poor photon emission rates, requiring photonic enhancement using resonant optical cavities. Moreover, many of the traditional hosts for erbium ions are not amenable to direct incorporation with existing integrated photonics platforms, limiting scalable fabrication of qubit-based devices. Here, we present a scalable approach toward CMOS-compatible telecom qubits by using erbium-doped titanium dioxide thin films grown atop silicon-on-insulator substrates. From this heterostructure, we have fabricated one-dimensional photonic crystal cavities demonstrating quality factors in excess of 5 × 10 4 and corresponding Purcell-enhanced optical emission rates of the erbium ensembles in excess of 200. This easily fabricated materials platform represents an important step toward realizing telecom quantum memories in a scalable qubit architecture compatible with mature silicon technologies.

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          Most cited references39

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          Quantum storage of photonic entanglement in a crystal

          Entanglement is the fundamental characteristic of quantum physics-much experimental effort is devoted to harnessing it between various physical systems. In particular, entanglement between light and material systems is interesting owing to their anticipated respective roles as 'flying' and stationary qubits in quantum information technologies (such as quantum repeaters and quantum networks). Here we report the demonstration of entanglement between a photon at a telecommunication wavelength (1,338 nm) and a single collective atomic excitation stored in a crystal. One photon from an energy-time entangled pair is mapped onto the crystal and then released into a well-defined spatial mode after a predetermined storage time. The other (telecommunication wavelength) photon is sent directly through a 50-metre fibre link to an analyser. Successful storage of entanglement in the crystal is proved by a violation of the Clauser-Horne-Shimony-Holt inequality by almost three standard deviations (S = 2.64 ± 0.23). These results represent an important step towards quantum communication technologies based on solid-state devices. In particular, our resources pave the way for building multiplexed quantum repeaters for long-distance quantum networks.
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            Optical quantum memory

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              Atomic Source of Single Photons in the Telecom Band

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                Author and article information

                Journal
                Nano Lett
                Nano Lett
                nl
                nalefd
                Nano Letters
                American Chemical Society
                1530-6984
                1530-6992
                08 August 2022
                24 August 2022
                : 22
                : 16
                : 6530-6536
                Affiliations
                []Nanoscience and Technology Division, Argonne National Laboratory , Lemont, Illinois 60439, United States
                []Center for Molecular Engineering, Argonne National Laboratory , Lemont, Illinois 60439, United States
                []Pritzker School of Molecular Engineering, University of Chicago , Chicago, Illinois 60637, United States
                [§ ]Materials Science Division, Argonne National Laboratory , Lemont, Illinois 60439, United States
                Author notes
                Author information
                https://orcid.org/0000-0001-5935-1364
                https://orcid.org/0000-0002-2716-668X
                https://orcid.org/0000-0002-5217-1069
                https://orcid.org/0000-0003-1173-343X
                https://orcid.org/0000-0002-8385-4882
                https://orcid.org/0000-0002-6843-5938
                https://orcid.org/0000-0002-3755-0044
                https://orcid.org/0000-0003-3337-7958
                https://orcid.org/0000-0001-5071-8318
                https://orcid.org/0000-0002-8591-2687
                Article
                10.1021/acs.nanolett.2c01561
                9413200
                35939762
                d879884d-a676-48fc-b67f-2f15d72df15c
                © 2022 UChicago Argonne, LLC, Operator of Argonne National Laboratory. Published by American Chemical Society

                Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works ( https://creativecommons.org/licenses/by-nc-nd/4.0/).

                History
                : 18 April 2022
                : 27 June 2022
                Funding
                Funded by: U.S. Department of Energy, doi 10.13039/100000015;
                Award ID: DE-FOA-0002253
                Categories
                Letter
                Custom metadata
                nl2c01561
                nl2c01561

                Nanotechnology
                purcell enhancement,rare earth ions,erbium,quantum optics
                Nanotechnology
                purcell enhancement, rare earth ions, erbium, quantum optics

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