Blackbody-sensitive room-temperature infrared photodetectors based on low-dimensional
      tellurium grown by chemical vapor deposition

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Abstract

Low-dimensional Te-based photodetectors exhibit blackbody response and achieve record-set performance metrics.

Abstract

Blackbody-sensitive room-temperature infrared detection is a notable development direction for future low-dimensional infrared photodetectors. However, because of the limitations of responsivity and spectral response range for low-dimensional narrow bandgap semiconductors, few low-dimensional infrared photodetectors exhibit blackbody sensitivity. Here, highly crystalline tellurium (Te) nanowires and two-dimensional nanosheets were synthesized by using chemical vapor deposition. The low-dimensional Te shows high hole mobility and broadband detection. The blackbody-sensitive infrared detection of Te devices was demonstrated. A high responsivity of 6650 A W ⁻¹ (at 1550-nm laser) and the blackbody responsivity of 5.19 A W ⁻¹ were achieved. High-resolution imaging based on Te photodetectors was successfully obtained. All the results suggest that the chemical vapor deposition–grown low-dimensional Te is one of the competitive candidates for sensitive focal-plane-array infrared photodetectors at room temperature.

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Author and article information

Journal

Journal ID (nlm-ta): Sci Adv

Journal ID (iso-abbrev): Sci Adv

Journal ID (publisher-id): SciAdv

Journal ID (hwp): advances

Title: Science Advances

Publisher: American Association for the Advancement of Science

ISSN (Electronic): 2375-2548

Publication date Collection: April 2021

Publication date (Electronic): 16 April 2021

Volume: 7

Issue: 16

Electronic Location Identifier: eabf7358

Affiliations

[1 ]State Key Laboratory of Infrared Physics, Shanghai Institute of Technical Physics Chinese Academy of Sciences, Shanghai 200083, China.

[2 ]Wuhan National Laboratory for Optoelectronics, Huazhong University of Science and Technology, Wuhan 430074, China.

[3 ]University of Chinese Academy of Sciences, Beijing 100049, China.

[4 ]Hangzhou Institute for Advanced Study, University of Chinese Academy of Sciences, Hangzhou 310024, China.

[5 ]Technical Center for Multifunctional Magneto-Optical Spectroscopy (Shanghai), Department of Materials, School of Physics and Electronic Science, East China Normal University, Shanghai, 200241, China.

[6 ]Department of Physics, State Key Laboratory of Surface Physics and Key Laboratory of Micro and Nano Photonic Structures (Ministry of Education), Fudan University, 200433 Shanghai, China.

[7 ]Henan Key Laboratory of Diamond Optoelectronic Materials and Devices, School of Physics and Engineering, Zhengzhou University, Zhengzhou 450001, China.

Author notes

[* ]Corresponding author. Email: wdhu@ 123456mail.sitp.ac.cn (W.H.); wangzhen@ 123456mail.sitp.ac.cn (Z.W.); w_peng@ 123456mail.sitp.ac.cn (P.W.); fwang@ 123456mail.sitp.ac.cn (F.W.)

[†]

These authors contributed equally to this work.

Author information

Meng Peng http://orcid.org/0000-0001-8301-5790

Runzhang Xie http://orcid.org/0000-0003-2389-9816

Zhen Wang http://orcid.org/0000-0002-7072-9003

Peng Wang http://orcid.org/0000-0002-7287-7595

Fang Wang http://orcid.org/0000-0002-3044-0571

Haonan Ge http://orcid.org/0000-0002-4597-404X

Yang Wang http://orcid.org/0000-0002-1024-3319

Fang Zhong http://orcid.org/0000-0002-0236-5578

Peisong Wu http://orcid.org/0000-0003-2264-7828

Jiafu Ye http://orcid.org/0000-0002-0576-5913

Qing Li http://orcid.org/0000-0003-2019-3156

Lili Zhang http://orcid.org/0000-0002-0440-5553

Xun Ge http://orcid.org/0000-0002-2668-408X

Yan Ye http://orcid.org/0000-0002-2838-1082

Yuchen Lei http://orcid.org/0000-0002-6646-5201

Wei Jiang http://orcid.org/0000-0002-8345-0853

Zhigao Hu http://orcid.org/0000-0003-0575-2191

Feng Wu http://orcid.org/0000-0003-0144-4423

Xiaohao Zhou http://orcid.org/0000-0002-5578-3183

Jinshui Miao http://orcid.org/0000-0002-3041-1105

Jianlu Wang http://orcid.org/0000-0002-0388-6148

Hugen Yan http://orcid.org/0000-0001-8423-6069

Chongxin Shan http://orcid.org/0000-0001-7119-5325

Jiangnan Dai http://orcid.org/0000-0002-0897-4534

Changqing Chen http://orcid.org/0000-0002-8853-9582

Xiaoshuang Chen http://orcid.org/0000-0003-0131-9454

Wei Lu http://orcid.org/0000-0001-9859-8394

Weida Hu http://orcid.org/0000-0001-5278-8969

Article

Publisher ID: abf7358

DOI: 10.1126/sciadv.abf7358

PMC ID: 8051875

PubMed ID: 33863732

SO-VID: 143eb268-c2c8-4c0c-922e-892bb147eaa2

Copyright © Copyright © 2021 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC).

License:

This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license, which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited.

History

Date received : 16 November 2020

Date accepted : 02 March 2021

Funding

Funded by: doi http://dx.doi.org/10.13039/100007219, Natural Science Foundation of Shanghai;

Award ID: 19XD1404100, 20YF1455900, 19YF1454600,18ZR1445900, 18ZR1445800

Funded by: doi http://dx.doi.org/10.13039/100007219, Natural Science Foundation of Shanghai;

Award ID: 19XD1404100

Funded by: doi http://dx.doi.org/10.13039/100007219, Natural Science Foundation of Shanghai;

Award ID: 20YF1455900

Funded by: doi http://dx.doi.org/10.13039/100007219, Natural Science Foundation of Shanghai;

Award ID: 19YF1454600

Funded by: doi http://dx.doi.org/10.13039/100007219, Natural Science Foundation of Shanghai;

Award ID: 18ZR1445900

Funded by: doi http://dx.doi.org/10.13039/100007219, Natural Science Foundation of Shanghai;

Award ID: 18ZR1445800