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      Subdiffractional focusing and guiding of polaritonic rays in a natural hyperbolic material

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          Abstract

          Uniaxial materials whose axial and tangential permittivities have opposite signs are referred to as indefinite or hyperbolic media. In such materials, light propagation is unusual leading to novel and often non-intuitive optical phenomena. Here we report infrared nano-imaging experiments demonstrating that crystals of hexagonal boron nitride, a natural mid-infrared hyperbolic material, can act as a ‘hyper-focusing lens' and as a multi-mode waveguide. The lensing is manifested by subdiffractional focusing of phonon–polaritons launched by metallic disks underneath the hexagonal boron nitride crystal. The waveguiding is revealed through the modal analysis of the periodic patterns observed around such launchers and near the sample edges. Our work opens new opportunities for anisotropic layered insulators in infrared nanophotonics complementing and potentially surpassing concurrent artificial hyperbolic materials with lower losses and higher optical localization.

          Abstract

          Hexagonal boron nitride has many interesting properties, including a natural hyperbolic dispersion, making it attractive for nanophotonic applications. Here, Dai et al. show that metallic disks under the material launch phonon–polaritons, turning it into a hyper-focusing lens.

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          Most cited references21

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          Van der Waals heterostructures

          Research on graphene and other two-dimensional atomic crystals is intense and likely to remain one of the hottest topics in condensed matter physics and materials science for many years. Looking beyond this field, isolated atomic planes can also be reassembled into designer heterostructures made layer by layer in a precisely chosen sequence. The first - already remarkably complex - such heterostructures (referred to as 'van der Waals') have recently been fabricated and investigated revealing unusual properties and new phenomena. Here we review this emerging research area and attempt to identify future directions. With steady improvement in fabrication techniques, van der Waals heterostructures promise a new gold rush, rather than a graphene aftershock.
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            Direct-bandgap properties and evidence for ultraviolet lasing of hexagonal boron nitride single crystal.

            The demand for compact ultraviolet laser devices is increasing, as they are essential in applications such as optical storage, photocatalysis, sterilization, ophthalmic surgery and nanosurgery. Many researchers are devoting considerable effort to finding materials with larger bandgaps than that of GaN. Here we show that hexagonal boron nitride (hBN) is a promising material for such laser devices because it has a direct bandgap in the ultraviolet region. We obtained a pure hBN single crystal under high-pressure and high-temperature conditions, which shows a dominant luminescence peak and a series of s-like exciton absorption bands around 215 nm, proving it to be a direct-bandgap material. Evidence for room-temperature ultraviolet lasing at 215 nm by accelerated electron excitation is provided by the enhancement and narrowing of the longitudinal mode, threshold behaviour of the excitation current dependence of the emission intensity, and a far-field pattern of the transverse mode.
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              Negative refraction makes a perfect lens

              With a conventional lens sharpness of the image is always limited by the wavelength of light. An unconventional alternative to a lens, a slab of negative refractive index material, has the power to focus all Fourier components of a 2D image, even those that do not propagate in a radiative manner. Such "superlenses" can be realized in the microwave band with current technology. Our simulations show that a version of the lens operating at the frequency of visible light can be realized in the form of a thin slab of silver. This optical version resolves objects only a few nanometers across.
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                Author and article information

                Journal
                Nat Commun
                Nat Commun
                Nature Communications
                Nature Pub. Group
                2041-1723
                22 April 2015
                : 6
                : 6963
                Affiliations
                [1 ]Department of Physics, University of California, San Diego , La Jolla, California 92093, USA
                [2 ]Department of Physics, Massachusetts Institute of Technology , Cambridge, Massachusetts 02215, USA
                [3 ]Department of Physics, Stony Brook University , Stony Brook, New York 11794, USA
                [4 ]National Institute for Materials Science, Namiki 1-1 , Tsukuba, Ibaraki 305-0044, Japan
                [5 ]Department of Chemistry and Biochemistry, University of California, San Diego , La Jolla, California 92093, USA
                [6 ]Ludwig-Maximilians-Universität and Center for Nanoscience , 80539 München, Germany
                Author notes
                Article
                ncomms7963
                10.1038/ncomms7963
                4421822
                25902364
                399fb4fc-689f-424b-a56f-fca886375118
                Copyright © 2015, Nature Publishing Group, a division of Macmillan Publishers Limited. All Rights Reserved.

                This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article's Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/

                History
                : 24 December 2014
                : 19 March 2015
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