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      Estimating the open biomass burning emissions in central and eastern China from 2003 to 2015 based on satellite observation

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          Abstract

          <p><strong>Abstract.</strong> Open biomass burning (OBB) has significant impacts on air pollution, climate change and potential human health. OBB has gathered wide attention but with little focus on the annual variation of pollutant emission. Central and eastern China (CEC) is one of the most polluted regions in China. This study aims to provide a state-of-the-art estimation of the pollutant emissions from OBB in CEC from 2003 to 2015, by adopting the satellite observation dataset – the burned area product (MCD64Al) and the active fire product (MCD14 ML) – along with local biomass data (updated biomass loading data and high-resolution vegetation data) and local emission factors. The successful adoption of the double satellite dataset for long-term estimation of pollutants from OBB with a high spatial resolution can support the assessing of OBB on regional air quality, especially for harvest periods or dry seasons. It is also useful to evaluate the effects of annual OBB management policies in different regions. Here, monthly emissions of pollutants were estimated and allocated into a 1×1<span class="thinspace"></span>km spatial grid for four types of OBB including grassland, shrubland, forest and cropland. From 2003 to 2015, the emissions from forest, shrubland and grassland fire burning had an annual fluctuation, whereas the emissions from crop straw burning steadily increased. The cumulative emissions of organic carbon (OC), elemental carbon (EC), methane (CH<sub>4</sub>), nitric oxide (NO<sub><i>x</i></sub>), non-methane volatile organic compounds (NMVOCs), sulfur dioxide (SO<sub>2</sub>), ammonia (NH<sub>3</sub>), carbon monoxide (CO), carbon dioxide (CO<sub>2</sub>) and fine particles (PM<sub>2.5</sub>) were 3.64×10<sup>3</sup>, 2.87×10<sup>2</sup>, 3.05×10<sup>3</sup>, 1.82×10<sup>3</sup>, 6.4×10<sup>3</sup>, 2.12×10<sup>2</sup>, 4.67×10<sup>2</sup>, 4.59×10<sup>4</sup>, 9.39×10<sup>5</sup> and 4.13×10<sup>3</sup><span class="thinspace"></span>Gg in these years, respectively. Crop straw burning was the largest contributor for all pollutant emissions, by 84<span class="thinspace"></span>%–96<span class="thinspace"></span>%. For the forest, shrubland and grassland fire burning, forest fire burning emissions contributed the most, and emissions from grassland fire were negligible due to little grass coverage in this region. High pollutant emissions concentrated in the connection area of Shandong, Henan, Jiangsu and Anhui, with emission intensity higher than 100 tons per square kilometer, which was related to the frequent agricultural activities in these regions. Peak emission of pollutants occurred during summer and autumn harvest periods including May, June, September and October, during which ∼ 50<span class="thinspace"></span>% of the total pollutant emissions were emitted in these months. This study highlights the importance of controlling the crop straw burning emissions. From December to March, the crop residue burning emissions decreased, while the emissions from forest, shrubland and grassland exhibited their highest values, leading to another small peak in emissions of pollutants. Obvious regional differences in seasonal variations of OBB were observed due to different local biomass types and environmental conditions. Rural population, agricultural output, economic levels, local burning habits, social customs and management policies were all influencing factors for OBB emissions.</p>

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          Most cited references63

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          Biomass burning in the tropics: impact on atmospheric chemistry and biogeochemical cycles.

          Biomass burning is widespread, especially in the tropics. It serves to clear land for shifting cultivation, to convert forests to agricultural and pastoral lands, and to remove dry vegetation in order to promote agricultural productivity and the growth of higher yield grasses. Furthermore, much agricultural waste and fuel wood is being combusted, particularly in developing countries. Biomass containing 2 to 5 petagrams of carbon is burned annually (1 petagram = 10(15) grams), producing large amounts of trace gases and aerosol particles that play important roles in atmospheric chemistry and climate. Emissions of carbon monoxide and methane by biomass burning affect the oxidation efficiency of the atmosphere by reacting with hydroxyl radicals, and emissions of nitric oxide and hydrocarbons lead to high ozone concentrations in the tropics during the dry season. Large quantities of smoke particles are produced as well, and these can serve as cloud condensation nuclei. These particles may thus substantially influence cloud microphysical and optical properties, an effect that could have repercussions for the radiation budget and the hydrological cycle in the tropics. Widespread burning may also disturb biogeochemical cycles, especially that of nitrogen. About 50 percent of the nitrogen in the biomass fuel can be released as molecular nitrogen. This pyrdenitrification process causes a sizable loss of fixed nitrogen in tropical ecosystems, in the range of 10 to 20 teragrams per year (1 teragram = 10(12) grams).
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            A technology-based global inventory of black and organic carbon emissions from combustion

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              Estimates of gross and net fluxes of carbon between the biosphere and the atmosphere from biomass burning

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                Author and article information

                Journal
                Atmospheric Chemistry and Physics
                Atmos. Chem. Phys.
                Copernicus GmbH
                1680-7324
                2018
                August 16 2018
                : 18
                : 16
                : 11623-11646
                Article
                10.5194/acp-18-11623-2018
                b51acceb-ed69-4dc7-9b6d-459bbb2404dd
                © 2018

                https://creativecommons.org/licenses/by/4.0/

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